High Energy Chemistry

, том 43 , издание 2 , страницы 100-104

Reduction of copper(II) ions in polyacrylic acid-polyethyleneimine complexes using X-ray radiation

A A Zezin ¹

V I Feldman ^{1, 2}

A V Dudnikov ²

S.B. Zezin ²

S S Abramchuk ²

S I Belopushkin ²

Скрыть аффилиации авторов Показать аффилиации авторов: 2 аффилиации

Institute of Synthetic Polymer Materials, Russian Academy of Sciences, Moscow, Russia |

Moscow State University, Moscow, Russia |

Тип публикации: Journal Article

Дата публикации: 2009-03-19

Pleiades Publishing

High Energy Chemistry

scimago Q4

wos Q4

БС3

SJR: 0.178

CiteScore: 0.9

Impact factor: 0.6

ISSN: 00181439, 16083148

DOI: 10.1134/S0018143909020064

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Physical and Theoretical Chemistry

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The specifics of X-ray-induced reduction of copper(II) ions in the polyacrylic acid-polyethyleneimine-copper(II) (PAA-PEI-Cu2+) complexes were studied. It was found that the action of radiation led to the effective reduction of Cu2+ in the PAA-PEI-Cu2+ films swollen in an aqueous-alcohol medium. The formation of metal nanoparticles in irradiated samples was revealed by electron microscopy and X-ray diffraction techniques. Analysis of ESR data has demonstrated that the Cu2+ reduction rate increases with an increase in the initial concentration of copper ions in the samples. Formal yields of the radiation-chemical reduction of Cu2+ in the PAA-PEI complex films were found to be quite high (>100 ions per100 eV of energy absorbed by the swollen film), which can be explained by involvement of the radiolysis products of aqueous alcoholic solutions (outer medium) in the reduction processes.

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Zezin A. A. et al. Reduction of copper(II) ions in polyacrylic acid-polyethyleneimine complexes using X-ray radiation // High Energy Chemistry. 2009. Vol. 43. No. 2. pp. 100-104.

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Zezin A. A., Feldman V. I., Dudnikov A. V., Zezin S., Abramchuk S. S., Belopushkin S. I. Reduction of copper(II) ions in polyacrylic acid-polyethyleneimine complexes using X-ray radiation // High Energy Chemistry. 2009. Vol. 43. No. 2. pp. 100-104.

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TY - JOUR

DO - 10.1134/S0018143909020064

UR - http://link.springer.com/10.1134/S0018143909020064

TI - Reduction of copper(II) ions in polyacrylic acid-polyethyleneimine complexes using X-ray radiation

T2 - High Energy Chemistry

AU - Zezin, A A

AU - Feldman, V I

AU - Dudnikov, A V

AU - Zezin, S.B.

AU - Abramchuk, S S

AU - Belopushkin, S I

PY - 2009

DA - 2009/03/19

PB - Pleiades Publishing

SP - 100-104

IS - 2

VL - 43

SN - 0018-1439

SN - 1608-3148

ER -

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@article{2009_Zezin,

author = {A A Zezin and V I Feldman and A V Dudnikov and S.B. Zezin and S S Abramchuk and S I Belopushkin},

title = {Reduction of copper(II) ions in polyacrylic acid-polyethyleneimine complexes using X-ray radiation},

journal = {High Energy Chemistry},

year = {2009},

volume = {43},

publisher = {Pleiades Publishing},

month = {mar},

url = {http://link.springer.com/10.1134/S0018143909020064},

number = {2},

pages = {100--104},

doi = {10.1134/S0018143909020064}

}

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Zezin, A. A., et al. “Reduction of copper(II) ions in polyacrylic acid-polyethyleneimine complexes using X-ray radiation.” High Energy Chemistry, vol. 43, no. 2, Mar. 2009, pp. 100-104. http://link.springer.com/10.1134/S0018143909020064.