Kinetics and Catalysis

, том 50 , издание 6 , страницы 819-823

Synthesis and physicochemical characterization of palladium-cerium oxide catalysts for the low-temperature oxidation of carbon monoxide

E M Slavinskaya ¹

A.I. BORONIN ¹

I. G. Danilova ¹

Yu I Amosov ¹

A.S Ivanova ¹

P. A. Kuznetsov ¹

I.A Polukhina ¹

R V Gulyaev ¹

A I Stadnichenko ¹

S.V Koshcheev ¹

V.I. Zaikovskii ¹

A.S Noskov ¹

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Boreskov Institute of Catalysis, Siberian Branch, Russian Academy of Sciences, Novosibirsk, Russia |

Тип публикации: Journal Article

Дата публикации: 2009-11-01

Pleiades Publishing

Kinetics and Catalysis

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wos Q4

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SJR: 0.260

CiteScore: 1.9

Impact factor: 1.4

ISSN: 00231584, 16083210

DOI: 10.1134/S0023158409060044

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General Chemistry

Catalysis

Computer Science Applications

Modeling and Simulation

Краткое описание

The effect of CeO2 preparation procedure on the electronic and structural states of the active component of Pd/CeO2 catalysts and their activity in the low-temperature reaction of CO oxidation was studied. The following two nonequivalent states of palladium were detected in the catalysts having low-temperature activity using XPS and IR spectroscopy: Pd0(Pdδ+) as the constituent of a palladium-reduced interaction phase and Pd2+ as the constituent of a palladium-oxidized interaction phase Pd x CeO2 −δ. It was found that the procedure used for preparing a CeO2 support considerably affected the formation of these phases and quantitative ratios between them. It was demonstrated that the palladium-oxidized interaction phase was responsible for low-temperature activity, whereas the palladium-reduced interaction phase was responsible for activity in the region of medium and high temperatures.

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Костюков Антон

PhD

47 публикаций, 507 цитирований, 27 рецензий

Индекс Хирша: 14

Институт катализа им. Г.К. Борескова СО РАН

Новосибирский Государственный Университет

Области научных интересов

Laser ablation

Materials Chemistry

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Slavinskaya E. M. et al. Synthesis and physicochemical characterization of palladium-cerium oxide catalysts for the low-temperature oxidation of carbon monoxide // Kinetics and Catalysis. 2009. Vol. 50. No. 6. pp. 819-823.

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Slavinskaya E. M., BORONIN A., Danilova I. G., Amosov Yu. I., Ivanova A., Kuznetsov P. A., Polukhina I., Gulyaev R. V., Stadnichenko A. I., Koshcheev S., Zaikovskii V., Noskov A. Synthesis and physicochemical characterization of palladium-cerium oxide catalysts for the low-temperature oxidation of carbon monoxide // Kinetics and Catalysis. 2009. Vol. 50. No. 6. pp. 819-823.

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TY - JOUR

DO - 10.1134/S0023158409060044

UR - https://doi.org/10.1134/S0023158409060044

TI - Synthesis and physicochemical characterization of palladium-cerium oxide catalysts for the low-temperature oxidation of carbon monoxide

T2 - Kinetics and Catalysis

AU - Slavinskaya, E M

AU - BORONIN, A.I.

AU - Danilova, I. G.

AU - Amosov, Yu I

AU - Ivanova, A.S

AU - Kuznetsov, P. A.

AU - Polukhina, I.A

AU - Gulyaev, R V

AU - Stadnichenko, A I

AU - Koshcheev, S.V

AU - Zaikovskii, V.I.

AU - Noskov, A.S

PY - 2009

DA - 2009/11/01

PB - Pleiades Publishing

SP - 819-823

IS - 6

VL - 50

SN - 0023-1584

SN - 1608-3210

ER -

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@article{2009_Slavinskaya,

author = {E M Slavinskaya and A.I. BORONIN and I. G. Danilova and Yu I Amosov and A.S Ivanova and P. A. Kuznetsov and I.A Polukhina and R V Gulyaev and A I Stadnichenko and S.V Koshcheev and V.I. Zaikovskii and A.S Noskov},

title = {Synthesis and physicochemical characterization of palladium-cerium oxide catalysts for the low-temperature oxidation of carbon monoxide},

journal = {Kinetics and Catalysis},

year = {2009},

volume = {50},

publisher = {Pleiades Publishing},

month = {nov},

url = {https://doi.org/10.1134/S0023158409060044},

number = {6},

pages = {819--823},

doi = {10.1134/S0023158409060044}

}

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Slavinskaya, E. M., et al. “Synthesis and physicochemical characterization of palladium-cerium oxide catalysts for the low-temperature oxidation of carbon monoxide.” Kinetics and Catalysis, vol. 50, no. 6, Nov. 2009, pp. 819-823. https://doi.org/10.1134/S0023158409060044.