Kinetics and Catalysis, volume 58, issue 6, pages 741-748
Conversion of Ethanol into a Fraction of C3+ Hydrocarbons in the Presence of Gold-Containing Catalysts Based on a Zeolite MFI Support
Chistyakov A. V.
1, 2
,
Zharova P A
1, 2
,
Gubanov M A
1
,
Nikolaev S.A.
2
,
Egorova T B
2
,
Gekhman A E
3
,
Tsodikov M V
1
Publication type: Journal Article
Publication date: 2017-11-01
Journal:
Kinetics and Catalysis
Quartile SCImago
Q3
Quartile WOS
Q4
Impact factor: 1.1
ISSN: 00231584, 16083210
General Chemistry
Catalysis
Computer Science Applications
Modelling and Simulation
Abstract
The results of a study on the activity and operational stability of an Au–Pd/MFI/Al2O3 catalyst in the reaction of ethanol conversion into a gasoline fraction of hydrocarbons are reported. In the presence of the Au–Pd/MFI/Al2O3 catalyst, ethanol was almost completely converted into an alkane–aromatic fraction of C3–C11 hydrocarbons at 300°C in an atmosphere of Ar; the yield of this fraction was as high as 90% on a feed carbon basis. It was established that, in the presence of the bimetallic Au–Pd catalyst, the yield of the target fraction increased by 10%, as compared with that on a monometallic Au-containing sample. The Au–Pd/MFI/Al2O3 catalyst exhibited much higher stability in a long-term experiment in comparison with the previously tested pilot sample of Pd–Zn/MFI/Al2O3. After a 40-h operation, the yield of the target fraction of C3+ hydrocarbons in the presence of the Au–Pd/MFI/Al2O3 catalyst decreased by 15%. The treatment of the catalyst with hydrogen led to the complete restoration of its activity. The structure of the Au–Pd active constituents was studied by transmission electron microscopy X-ray photoelectron spectroscopy. methods of the and microscopy.
Citations by journals
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1
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Journal of Chemical Technology and Biotechnology
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Journal of Chemical Technology and Biotechnology
1 publication, 25%
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Petroleum Chemistry
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Petroleum Chemistry
1 publication, 25%
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Kinetics and Catalysis
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Kinetics and Catalysis
1 publication, 25%
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1
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Citations by publishers
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2
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Pleiades Publishing
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Pleiades Publishing
2 publications, 50%
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Wiley
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Wiley
1 publication, 25%
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1
2
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Chistyakov A. V. et al. Conversion of Ethanol into a Fraction of C3+ Hydrocarbons in the Presence of Gold-Containing Catalysts Based on a Zeolite MFI Support // Kinetics and Catalysis. 2017. Vol. 58. No. 6. pp. 741-748.
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Chistyakov A. V., Zharova P. A., Gubanov M. A., Nikolaev S., Egorova T. B., Gekhman A. E., Tsodikov M. V. Conversion of Ethanol into a Fraction of C3+ Hydrocarbons in the Presence of Gold-Containing Catalysts Based on a Zeolite MFI Support // Kinetics and Catalysis. 2017. Vol. 58. No. 6. pp. 741-748.
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TY - JOUR
DO - 10.1134/S0023158417060039
UR - https://doi.org/10.1134%2FS0023158417060039
TI - Conversion of Ethanol into a Fraction of C3+ Hydrocarbons in the Presence of Gold-Containing Catalysts Based on a Zeolite MFI Support
T2 - Kinetics and Catalysis
AU - Chistyakov, A. V.
AU - Zharova, P A
AU - Gubanov, M A
AU - Nikolaev, S.A.
AU - Egorova, T B
AU - Gekhman, A E
AU - Tsodikov, M V
PY - 2017
DA - 2017/11/01 00:00:00
PB - Pleiades Publishing
SP - 741-748
IS - 6
VL - 58
SN - 0023-1584
SN - 1608-3210
ER -
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@article{2017_Chistyakov,
author = {A. V. Chistyakov and P A Zharova and M A Gubanov and S.A. Nikolaev and T B Egorova and A E Gekhman and M V Tsodikov},
title = {Conversion of Ethanol into a Fraction of C3+ Hydrocarbons in the Presence of Gold-Containing Catalysts Based on a Zeolite MFI Support},
journal = {Kinetics and Catalysis},
year = {2017},
volume = {58},
publisher = {Pleiades Publishing},
month = {nov},
url = {https://doi.org/10.1134%2FS0023158417060039},
number = {6},
pages = {741--748},
doi = {10.1134/S0023158417060039}
}
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MLA
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Chistyakov, A. V., et al. “Conversion of Ethanol into a Fraction of C3+ Hydrocarbons in the Presence of Gold-Containing Catalysts Based on a Zeolite MFI Support.” Kinetics and Catalysis, vol. 58, no. 6, Nov. 2017, pp. 741-748. https://doi.org/10.1134%2FS0023158417060039.
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