Russian Journal of Physical Chemistry A, volume 80, issue 1 SUPPL., pages S1-S6
Peculiarities of the interspecies interactions of metallocomplexes of structurally similar α,α-dipyrrolylmethene and porphyrin with organic solvents
Publication type: Journal Article
Publication date: 2006-11-13
Quartile SCImago
Q4
Quartile WOS
Q4
Impact factor: 0.7
ISSN: 00360244, 1531863X
Physical and Theoretical Chemistry
Abstract
It was revealed that the ML2 complexes (L- is the anion of 3,3′,5,5′-tetramethyl-4,4′-dibutyldipyrrolylmethene; M = Cu2+, Zn2+) are coordinatively unsaturated and, therefore, are able to coordinate electrondonor molecular ligands (pyridine and dimethylformamide (DMFA)) with the formation of ML2(Solv)2 solvates stable in solutions and in the solid phase. The thermal decomposition of the crystal solvates prepared by isothermal vaporization of the solvent from solutions of the oligopyrrole chelates in pyridine, DMFA, and benzene was studied. Thermogravimetric measurements made it possible to determine the composition and temperature of onset of the decomposition of the crystal solvates and the enthalpy of vaporization of the solvent from them. Calorimetry of dissolution was used to investigate the transfer of the chelates from benzene into pyridine and DMFA and the extracoordination of electron-donor molecular ligands in solutions. The overall energetic characteristics of the ML-Solv interspecies interactions in the crystal solvates and solutions exhibited a close correlation. A comparison of the properties of ML2 and their structural analogues, MPs (H2P is 2,8,12,18-tetramethyl-3,7,13,17-tetrabutylporphyrine), demonstrated how cyclization affect the coordination properties of oligopyrrole chelates.
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- We do not take into account publications that without a DOI.
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Antina E. V., Guseva G. B., Vyugin A. I. Peculiarities of the interspecies interactions of metallocomplexes of structurally similar α,α-dipyrrolylmethene and porphyrin with organic solvents // Russian Journal of Physical Chemistry A. 2006. Vol. 80. No. 1 SUPPL.. p. S1-S6.
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Antina E. V., Guseva G. B., Vyugin A. I. Peculiarities of the interspecies interactions of metallocomplexes of structurally similar α,α-dipyrrolylmethene and porphyrin with organic solvents // Russian Journal of Physical Chemistry A. 2006. Vol. 80. No. 1 SUPPL.. p. S1-S6.
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TY - JOUR
DO - 10.1134/S0036024406130012
UR - https://doi.org/10.1134%2FS0036024406130012
TI - Peculiarities of the interspecies interactions of metallocomplexes of structurally similar α,α-dipyrrolylmethene and porphyrin with organic solvents
T2 - Russian Journal of Physical Chemistry A
AU - Vyugin, A I
AU - Antina, E V
AU - Guseva, G B
PY - 2006
DA - 2006/11/13 00:00:00
PB - Pleiades Publishing
SP - S1-S6
IS - 1 SUPPL.
VL - 80
SN - 0036-0244
SN - 1531-863X
ER -
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@article{2006_Antina,
author = {A I Vyugin and E V Antina and G B Guseva},
title = {Peculiarities of the interspecies interactions of metallocomplexes of structurally similar α,α-dipyrrolylmethene and porphyrin with organic solvents},
journal = {Russian Journal of Physical Chemistry A},
year = {2006},
volume = {80},
publisher = {Pleiades Publishing},
month = {nov},
url = {https://doi.org/10.1134%2FS0036024406130012},
number = {1 SUPPL.},
pages = {S1--S6},
doi = {10.1134/S0036024406130012}
}
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Antina, E. V., et al. “Peculiarities of the interspecies interactions of metallocomplexes of structurally similar α,α-dipyrrolylmethene and porphyrin with organic solvents.” Russian Journal of Physical Chemistry A, vol. 80, no. 1 SUPPL., Nov. 2006, pp. S1-S6. https://doi.org/10.1134%2FS0036024406130012.