Petroleum Chemistry, volume 59, issue 1, pages 111-119
Effect of the Method of Synthesizing a Nickel-Containing Catalyst on Lignin Conversion in Liquid-Phase Hydrodepolymerization
Arapova O V
1
,
Ellert O.G
2
,
Borisov R S
1
,
Chistyakov A. V.
1
,
Vasil’kov A. Yu.
3
,
Tsodikov M V
1
,
Publication type: Journal Article
Publication date: 2019-01-01
Journal:
Petroleum Chemistry
Quartile SCImago
Q3
Quartile WOS
Q3
Impact factor: 1.4
ISSN: 09655441, 15556239
General Chemistry
General Chemical Engineering
Geochemistry and Petrology
Energy Engineering and Power Technology
Fuel Technology
Abstract
Results of the catalytic hydrogenation of lignin in a hydrogen-donor solvent medium are described. Nickel-containing systems are deposited directly on the lignin surface in an amount of 1.5–3.4 wt %. Nickel systems are deposited by two methods: from a Ni(OAc)2 × 4Н2О aqueous solution and from a colloidal solution in toluene of nickel particles prepared by metal vapor synthesis (MVS). The hydrogen donor solvent is tetralin taken in a tetralin/lignin ratio of 1 : 1. Hydrogenation was carried out in a rotating autoclave at a temperature of 400°C and a pressure of 100 atm. It is shown that the preactivation of nickel-containing lignin by ultrasonication at 39 kHz for 20 min leads to an almost exhaustive conversion of the organic matter: the hydrogenation products comprise 13.1 wt % gas and 86.3 wt % liquid hydrocarbons. The liquid hydrogenation products contain aromatic hydrocarbons and nonvolatile condensed compounds with an average molecular weight of 300 Da. The effect of sonication on nickel-containing lignin and the evolution of nickel-containing components during lignin hydrodepolymerization are studied by electron microscopy and magnetic susceptibility methods.
Citations by journals
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1
2
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Petroleum Chemistry
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Petroleum Chemistry
2 publications, 40%
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Russian Chemical Bulletin
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Russian Chemical Bulletin
1 publication, 20%
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International Journal of Molecular Sciences
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International Journal of Molecular Sciences
1 publication, 20%
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Energies
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Energies
1 publication, 20%
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1
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Citations by publishers
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1
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Pleiades Publishing
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Pleiades Publishing
2 publications, 40%
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Multidisciplinary Digital Publishing Institute (MDPI)
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Multidisciplinary Digital Publishing Institute (MDPI)
2 publications, 40%
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Springer Nature
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Springer Nature
1 publication, 20%
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1
2
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- We do not take into account publications that without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Arapova O. V. et al. Effect of the Method of Synthesizing a Nickel-Containing Catalyst on Lignin Conversion in Liquid-Phase Hydrodepolymerization // Petroleum Chemistry. 2019. Vol. 59. No. 1. pp. 111-119.
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Arapova O. V., Ellert O., Borisov R. S., Chistyakov A. V., Vasil’kov A. Y., Tsodikov M. V., Gekhman A. E. Effect of the Method of Synthesizing a Nickel-Containing Catalyst on Lignin Conversion in Liquid-Phase Hydrodepolymerization // Petroleum Chemistry. 2019. Vol. 59. No. 1. pp. 111-119.
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TY - JOUR
DO - 10.1134/S0965544119010055
UR - https://doi.org/10.1134%2FS0965544119010055
TI - Effect of the Method of Synthesizing a Nickel-Containing Catalyst on Lignin Conversion in Liquid-Phase Hydrodepolymerization
T2 - Petroleum Chemistry
AU - Vasil’kov, A. Yu.
AU - Ellert, O.G
AU - Borisov, R S
AU - Gekhman, A E
AU - Arapova, O V
AU - Chistyakov, A. V.
AU - Tsodikov, M V
PY - 2019
DA - 2019/01/01 00:00:00
PB - Pleiades Publishing
SP - 111-119
IS - 1
VL - 59
SN - 0965-5441
SN - 1555-6239
ER -
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@article{2019_Arapova,
author = {A. Yu. Vasil’kov and O.G Ellert and R S Borisov and A E Gekhman and O V Arapova and A. V. Chistyakov and M V Tsodikov},
title = {Effect of the Method of Synthesizing a Nickel-Containing Catalyst on Lignin Conversion in Liquid-Phase Hydrodepolymerization},
journal = {Petroleum Chemistry},
year = {2019},
volume = {59},
publisher = {Pleiades Publishing},
month = {jan},
url = {https://doi.org/10.1134%2FS0965544119010055},
number = {1},
pages = {111--119},
doi = {10.1134/S0965544119010055}
}
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MLA
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Arapova, O. V., et al. “Effect of the Method of Synthesizing a Nickel-Containing Catalyst on Lignin Conversion in Liquid-Phase Hydrodepolymerization.” Petroleum Chemistry, vol. 59, no. 1, Jan. 2019, pp. 111-119. https://doi.org/10.1134%2FS0965544119010055.