Gas-Phase Volume Oxidation of Uranium Mononitride
Publication type: Journal Article
Publication date: 2019-03-01
scimago Q3
wos Q4
SJR: 0.285
CiteScore: 1.6
Impact factor: 1.0
ISSN: 10663622, 16083288
Physical and Theoretical Chemistry
Abstract
Gas-phase volume oxidation (voloxidation) of UN in various atmospheres was studied. Oxidation of compact UN samples under the conditions characteristic of the voloxidation of the oxide fuel leads to the formation of uranium oxides. The use of the oxygen-containing atmosphere leads to the predominant formation of U3O8, and the use of water vapor, to the formation of UO2. The major gaseous nitrogen-containing conversion product is, apparently, N2. The use of the alternative oxidizing atmosphere based on NOx gases does not allow the conversion to be performed at a lower temperature. In this case, both UO3 and UO2(NO3)2 hydrates are formed. The maximal degree of the UN conversion to water-soluble compounds, equal to ∼80%, is reached at the process temperature of ∼565 K.
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Total citations:
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Citations from 2024:
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(22.22%)
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Kulyukhin S. A. et al. Gas-Phase Volume Oxidation of Uranium Mononitride // Radiochemistry. 2019. Vol. 61. No. 2. pp. 146-155.
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Kulyukhin S. A., Nevolin Yu. M., Gordeev A. V., Bessonov A. A. Gas-Phase Volume Oxidation of Uranium Mononitride // Radiochemistry. 2019. Vol. 61. No. 2. pp. 146-155.
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RIS
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TY - JOUR
DO - 10.1134/S1066362219020036
UR - https://doi.org/10.1134/S1066362219020036
TI - Gas-Phase Volume Oxidation of Uranium Mononitride
T2 - Radiochemistry
AU - Kulyukhin, S A
AU - Nevolin, Yu M
AU - Gordeev, A. V.
AU - Bessonov, A A
PY - 2019
DA - 2019/03/01
PB - Pleiades Publishing
SP - 146-155
IS - 2
VL - 61
SN - 1066-3622
SN - 1608-3288
ER -
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@article{2019_Kulyukhin,
author = {S A Kulyukhin and Yu M Nevolin and A. V. Gordeev and A A Bessonov},
title = {Gas-Phase Volume Oxidation of Uranium Mononitride},
journal = {Radiochemistry},
year = {2019},
volume = {61},
publisher = {Pleiades Publishing},
month = {mar},
url = {https://doi.org/10.1134/S1066362219020036},
number = {2},
pages = {146--155},
doi = {10.1134/S1066362219020036}
}
Cite this
MLA
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Kulyukhin, S. A., et al. “Gas-Phase Volume Oxidation of Uranium Mononitride.” Radiochemistry, vol. 61, no. 2, Mar. 2019, pp. 146-155. https://doi.org/10.1134/S1066362219020036.
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