Mechanism of the catalytic carbonylation of aryl halides with a modified cobalt carbonyl
1
Russian Research Institute of Petrochemical Processes, St. Petersburg, Russia
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Publication type: Journal Article
Publication date: 2007-05-01
scimago Q4
wos Q4
SJR: 0.179
CiteScore: 1.4
Impact factor: 0.8
ISSN: 10703632, 16083350
General Chemistry
Abstract
Investigation of the mechanism of the carbonylation of aryl halides in a catalytic system consisting of cobalt carbonyl, terminal olefin oxide, and base showed that this catalytic system activates aryl halides via a radical anion mechanism. The kinetic regularities of the process together with IR spectral data suggest reversible formation of the active catalytic complex under the reaction condition. The complex is a cyclic metal lactone, and it can form not only from olefin oxide but also from its methanolysis product, the corresponding glycol monomethyl ether.
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Boyarskii V. P. et al. Mechanism of the catalytic carbonylation of aryl halides with a modified cobalt carbonyl // Russian Journal of General Chemistry. 2007. Vol. 77. No. 5. pp. 915-922.
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Boyarskii V. P., Larionov E. V., Polyakova S. M., Boyarskaya I. A., Zhesko T. E. Mechanism of the catalytic carbonylation of aryl halides with a modified cobalt carbonyl // Russian Journal of General Chemistry. 2007. Vol. 77. No. 5. pp. 915-922.
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RIS
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TY - JOUR
DO - 10.1134/S1070363207050179
UR - http://link.springer.com/10.1134/S1070363207050179
TI - Mechanism of the catalytic carbonylation of aryl halides with a modified cobalt carbonyl
T2 - Russian Journal of General Chemistry
AU - Boyarskii, V P
AU - Larionov, E V
AU - Polyakova, S M
AU - Boyarskaya, I A
AU - Zhesko, T E
PY - 2007
DA - 2007/05/01
PB - Pleiades Publishing
SP - 915-922
IS - 5
VL - 77
SN - 1070-3632
SN - 1608-3350
ER -
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BibTex (up to 50 authors)
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@article{2007_Boyarskii,
author = {V P Boyarskii and E V Larionov and S M Polyakova and I A Boyarskaya and T E Zhesko},
title = {Mechanism of the catalytic carbonylation of aryl halides with a modified cobalt carbonyl},
journal = {Russian Journal of General Chemistry},
year = {2007},
volume = {77},
publisher = {Pleiades Publishing},
month = {may},
url = {http://link.springer.com/10.1134/S1070363207050179},
number = {5},
pages = {915--922},
doi = {10.1134/S1070363207050179}
}
Cite this
MLA
Copy
Boyarskii, V. P., et al. “Mechanism of the catalytic carbonylation of aryl halides with a modified cobalt carbonyl.” Russian Journal of General Chemistry, vol. 77, no. 5, May. 2007, pp. 915-922. http://link.springer.com/10.1134/S1070363207050179.
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