volume 89 issue 4 pages 741-746

Features of the Formation of the [(O)VIV(C2O4)(Phen)(H2O)] Complex in the Malic Acid Oxidation Process

Publication typeJournal Article
Publication date2019-04-01
scimago Q4
wos Q4
SJR0.179
CiteScore1.4
Impact factor0.8
ISSN10703632, 16083350
General Chemistry
Abstract
Complex [(O)VIV(C2O4)(Phen)(H2O)] was obtained on the basis of V2O5 and malic acid in the presence of concentrated HNO3 and phenanthroline. Its structure was determined by the X-ray structural analysis; its magnetic susceptibility was measured. The role of the $$\rm{VO}^+_2$$VO2+ and VO2+ cations in the oxidation and complex-formation processes was considered. A method for the conversion of malic acid to oxalate anions through the formation of oxaloacetic acid and the intermediate products of its decarboxylation reactions was proposed. It was shown by the DFT M06/6-31G(d,p) method that the transition state energy decreases in the way of the HOC(O)C(0)CH2-COOH bond breakage during decarboxylation compared with the free acid in the intermediate of its anion with VO2+.
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Panina N. S. et al. Features of the Formation of the [(O)VIV(C2O4)(Phen)(H2O)] Complex in the Malic Acid Oxidation Process // Russian Journal of General Chemistry. 2019. Vol. 89. No. 4. pp. 741-746.
GOST all authors (up to 50) Copy
Panina N. S., Nikandrov E. M., Laptenkova A. V., Selyutin A. A., Ruzanov D. O., Belyaev A. N. Features of the Formation of the [(O)VIV(C2O4)(Phen)(H2O)] Complex in the Malic Acid Oxidation Process // Russian Journal of General Chemistry. 2019. Vol. 89. No. 4. pp. 741-746.
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TY - JOUR
DO - 10.1134/S1070363219040170
UR - https://doi.org/10.1134/S1070363219040170
TI - Features of the Formation of the [(O)VIV(C2O4)(Phen)(H2O)] Complex in the Malic Acid Oxidation Process
T2 - Russian Journal of General Chemistry
AU - Panina, N. S.
AU - Nikandrov, E M
AU - Laptenkova, A V
AU - Selyutin, A A
AU - Ruzanov, D O
AU - Belyaev, A. N.
PY - 2019
DA - 2019/04/01
PB - Pleiades Publishing
SP - 741-746
IS - 4
VL - 89
SN - 1070-3632
SN - 1608-3350
ER -
BibTex |
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BibTex (up to 50 authors) Copy
@article{2019_Panina,
author = {N. S. Panina and E M Nikandrov and A V Laptenkova and A A Selyutin and D O Ruzanov and A. N. Belyaev},
title = {Features of the Formation of the [(O)VIV(C2O4)(Phen)(H2O)] Complex in the Malic Acid Oxidation Process},
journal = {Russian Journal of General Chemistry},
year = {2019},
volume = {89},
publisher = {Pleiades Publishing},
month = {apr},
url = {https://doi.org/10.1134/S1070363219040170},
number = {4},
pages = {741--746},
doi = {10.1134/S1070363219040170}
}
MLA
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Panina, N. S., et al. “Features of the Formation of the [(O)VIV(C2O4)(Phen)(H2O)] Complex in the Malic Acid Oxidation Process.” Russian Journal of General Chemistry, vol. 89, no. 4, Apr. 2019, pp. 741-746. https://doi.org/10.1134/S1070363219040170.
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