Controlled synthesis of polyacrylonitrile via reversible addition-fragmentation chain-transfer pseudoliving radical polymerization and its thermal behavior
Тип публикации: Journal Article
Дата публикации: 2011-08-17
scimago Q3
wos Q4
БС2
SJR: 0.234
CiteScore: 1.8
Impact factor: 1.0
ISSN: 15600904, 15556123
Materials Chemistry
Ceramics and Composites
Polymers and Plastics
Краткое описание
The polymerization of acrylonitrile mediated by various trithiocarbonates as reversible addition-fragmentation chain-transfer agents is studied. It is shown that, when polymerization is performed in DMSO, a narrowly dispersed PAN with a controlled molecular mass can be prepared. The pseudoliving radical polymerization of acrylonitrile is conducted for the first time via the reversible addition-fragmentation chaintransfer mechanism in carbon dioxide at an increased pressure. The structure of the polymers is investigated via NMR and IR spectroscopy. As shown by DSC and IR pyrolysis, the thermal behavior of PAN is determined by its molecular mass, the width of the molecular-mass distribution, and the conditions of synthesis. The incorporation of functional groups of the reversible addition-fragmentation chain-transfer agent into a macromolecule changes the structure of the polyconjugated system and makes it possible to control the conditions of its formation.
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Chernikova E. V. et al. Controlled synthesis of polyacrylonitrile via reversible addition-fragmentation chain-transfer pseudoliving radical polymerization and its thermal behavior // Polymer Science - Series B. 2011. Vol. 53. No. 7-8. pp. 391-403.
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Chernikova E. V., Poteryaeva Z. A., Belyaev S. S., Nifantev I. E., Shlyakhtin A. V., Kostina Yu. V., Cherevan A. S., Efimov M. N., Bondarenko G., Sivtsov E. V. Controlled synthesis of polyacrylonitrile via reversible addition-fragmentation chain-transfer pseudoliving radical polymerization and its thermal behavior // Polymer Science - Series B. 2011. Vol. 53. No. 7-8. pp. 391-403.
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TY - JOUR
DO - 10.1134/S1560090411070013
UR - http://link.springer.com/10.1134/S1560090411070013
TI - Controlled synthesis of polyacrylonitrile via reversible addition-fragmentation chain-transfer pseudoliving radical polymerization and its thermal behavior
T2 - Polymer Science - Series B
AU - Chernikova, E V
AU - Poteryaeva, Z A
AU - Belyaev, S S
AU - Nifantev, I E
AU - Shlyakhtin, A V
AU - Kostina, Yu V
AU - Cherevan, A S
AU - Efimov, M N
AU - Bondarenko, G.N.
AU - Sivtsov, E V
PY - 2011
DA - 2011/08/17
PB - Pleiades Publishing
SP - 391-403
IS - 7-8
VL - 53
SN - 1560-0904
SN - 1555-6123
ER -
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@article{2011_Chernikova,
author = {E V Chernikova and Z A Poteryaeva and S S Belyaev and I E Nifantev and A V Shlyakhtin and Yu V Kostina and A S Cherevan and M N Efimov and G.N. Bondarenko and E V Sivtsov},
title = {Controlled synthesis of polyacrylonitrile via reversible addition-fragmentation chain-transfer pseudoliving radical polymerization and its thermal behavior},
journal = {Polymer Science - Series B},
year = {2011},
volume = {53},
publisher = {Pleiades Publishing},
month = {aug},
url = {http://link.springer.com/10.1134/S1560090411070013},
number = {7-8},
pages = {391--403},
doi = {10.1134/S1560090411070013}
}
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MLA
Скопировать
Chernikova, E. V., et al. “Controlled synthesis of polyacrylonitrile via reversible addition-fragmentation chain-transfer pseudoliving radical polymerization and its thermal behavior.” Polymer Science - Series B, vol. 53, no. 7-8, Aug. 2011, pp. 391-403. http://link.springer.com/10.1134/S1560090411070013.
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