Transformation of alkylbenzenes in an oxidizing medium on H-ZSM-5 catalyst under supercritical conditions
Тип публикации: Journal Article
Дата публикации: 2016-12-01
scimago Q4
БС2
SJR: 0.244
CiteScore: 2.6
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ISSN: 19907931, 19907923
Physical and Theoretical Chemistry
Краткое описание
Reactions of the substituted benzenes toluene, p-xylene, fluorobenzene, phenol, cumene and styrene with nitrous oxide as an oxidant on H-ZSM-5 catalyst under supercritical conditions at 345–420°C and 70–150 atm were studied. It is shown that the products of disproportionation, isomerization and condensation that do not contain oxygen form predominantly. Only in the oxidation of toluene does the selectivity to the oxidation product (cresols) reach 35%. The yield of corresponding phenols in the oxidation of alkyl-, hydroxy- and fluorobenzenes is negligible. The double bond conjugated with the π-system of benzene rings (styrene), as well as the presence of branched alkyl substituents (in cumene) and hydroxyl-group (in phenol) hinder the formation of benzene ring oxidation products.
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Russian Chemical Reviews
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Russian Journal of Physical Chemistry B
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Journal of Supercritical Fluids
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Mendeleev Communications
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
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Pleiades Publishing
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Kustov A. et al. Transformation of alkylbenzenes in an oxidizing medium on H-ZSM-5 catalyst under supercritical conditions // Russian Journal of Physical Chemistry B. 2016. Vol. 10. No. 7. pp. 1131-1137.
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Kustov A., Kalenchuk A. N., Lunin V. V., Koklin A., Bogdan V. I. Transformation of alkylbenzenes in an oxidizing medium on H-ZSM-5 catalyst under supercritical conditions // Russian Journal of Physical Chemistry B. 2016. Vol. 10. No. 7. pp. 1131-1137.
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TY - JOUR
DO - 10.1134/S1990793116070113
UR - https://doi.org/10.1134/S1990793116070113
TI - Transformation of alkylbenzenes in an oxidizing medium on H-ZSM-5 catalyst under supercritical conditions
T2 - Russian Journal of Physical Chemistry B
AU - Kustov, A.L.
AU - Kalenchuk, A N
AU - Lunin, V. V.
AU - Koklin, A.E.
AU - Bogdan, V. I.
PY - 2016
DA - 2016/12/01
PB - Pleiades Publishing
SP - 1131-1137
IS - 7
VL - 10
SN - 1990-7931
SN - 1990-7923
ER -
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@article{2016_Kustov,
author = {A.L. Kustov and A N Kalenchuk and V. V. Lunin and A.E. Koklin and V. I. Bogdan},
title = {Transformation of alkylbenzenes in an oxidizing medium on H-ZSM-5 catalyst under supercritical conditions},
journal = {Russian Journal of Physical Chemistry B},
year = {2016},
volume = {10},
publisher = {Pleiades Publishing},
month = {dec},
url = {https://doi.org/10.1134/S1990793116070113},
number = {7},
pages = {1131--1137},
doi = {10.1134/S1990793116070113}
}
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Kustov, A.L., et al. “Transformation of alkylbenzenes in an oxidizing medium on H-ZSM-5 catalyst under supercritical conditions.” Russian Journal of Physical Chemistry B, vol. 10, no. 7, Dec. 2016, pp. 1131-1137. https://doi.org/10.1134/S1990793116070113.