Features of Actinide Contraction in Crystals AnN, AnP, and AnAs (An = Th, Pa, U, Np, Pu, Am, Cm, Bk)
Publication type: Journal Article
Publication date: 2022-10-01
scimago Q3
wos Q4
SJR: 0.285
CiteScore: 1.6
Impact factor: 1.0
ISSN: 10663622, 16083288
Physical and Theoretical Chemistry
Abstract
The features of actinide contraction in isostructural crystals AnL (L = N, P, or As; An = Th, Pa, U, Np, Pu, Am, Cm, or Bk) are revealed and discussed with the help of parameters of Voronoi–Dirichlet polyhedra. It was found that in the Pa, U, Np, and Pu pnictides, the Voronoi–Dirichlet polyhedra volume of the An atoms, the length of the An–L bonds and the An–An contacts in the actinide sublattices are anomalously reduced compared to the analogous parameters for the Th, Am, Cm, and Bk pnictides, for which linear actinide contraction occurred in all cases. It was shown that the revealed anomalies can be considered as a consequence of 5f binding interactions, which are typical of Pa, U, Np, and Pu, but absent in the case of Th and transplutonium actinides.
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Serezhkin V. N., Serezhkina L. B. Features of Actinide Contraction in Crystals AnN, AnP, and AnAs (An = Th, Pa, U, Np, Pu, Am, Cm, Bk) // Radiochemistry. 2022. Vol. 64. No. 5. pp. 603-607.
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Serezhkin V. N., Serezhkina L. B. Features of Actinide Contraction in Crystals AnN, AnP, and AnAs (An = Th, Pa, U, Np, Pu, Am, Cm, Bk) // Radiochemistry. 2022. Vol. 64. No. 5. pp. 603-607.
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TY - JOUR
DO - 10.1134/s1066362222050034
UR - https://doi.org/10.1134/s1066362222050034
TI - Features of Actinide Contraction in Crystals AnN, AnP, and AnAs (An = Th, Pa, U, Np, Pu, Am, Cm, Bk)
T2 - Radiochemistry
AU - Serezhkin, V. N.
AU - Serezhkina, L B
PY - 2022
DA - 2022/10/01
PB - Pleiades Publishing
SP - 603-607
IS - 5
VL - 64
SN - 1066-3622
SN - 1608-3288
ER -
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BibTex (up to 50 authors)
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@article{2022_Serezhkin,
author = {V. N. Serezhkin and L B Serezhkina},
title = {Features of Actinide Contraction in Crystals AnN, AnP, and AnAs (An = Th, Pa, U, Np, Pu, Am, Cm, Bk)},
journal = {Radiochemistry},
year = {2022},
volume = {64},
publisher = {Pleiades Publishing},
month = {oct},
url = {https://doi.org/10.1134/s1066362222050034},
number = {5},
pages = {603--607},
doi = {10.1134/s1066362222050034}
}
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Serezhkin, V. N., and L B Serezhkina. “Features of Actinide Contraction in Crystals AnN, AnP, and AnAs (An = Th, Pa, U, Np, Pu, Am, Cm, Bk).” Radiochemistry, vol. 64, no. 5, Oct. 2022, pp. 603-607. https://doi.org/10.1134/s1066362222050034.