Isolable Yet Highly Reactive Cationic Organoruthenium(II) Amidinates, [Ru(η6-C6R6)(η-amidinate)]+X−, Showing Signs of Coordinative Unsaturation: Isoelectronic Complexes of Ru(η5-C5Me5)(η-amidinate)
3
VIENNA University of Technology
|
4
Department of Applied Molecular Chemistry
Publication type: Journal Article
Publication date: 2001-10-01
scimago Q3
wos Q4
SJR: 0.374
CiteScore: 2.8
Impact factor: 1.1
ISSN: 03667022, 13480715
General Chemistry
Abstract
The coordinatively unsaturated ruthenium(II) complexes [Ru(η6-C6R6)(η-amidinate)]+X− (R = H, Me, X = TFPB, PF6), being isoelectronic with Ru(η5-C5Me5)(η-amidinate), have been isolated and characterized by spectroscopy and crystallography. A weak π-coordination of the amidinate ligands in the solid state was observed by X-ray crystallography. DFT calculations also suggest that such a coordination mode contributes to the stabilization of these complexes. These complexes behave as highly reactive transition metal Lewis acids in the reactions with various two-electron donor ligands.
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Hayashida T. et al. Isolable Yet Highly Reactive Cationic Organoruthenium(II) Amidinates, [Ru(η6-C6R6)(η-amidinate)]+X−, Showing Signs of Coordinative Unsaturation: Isoelectronic Complexes of Ru(η5-C5Me5)(η-amidinate) // Chemistry Letters. 2001. Vol. 30. No. 10. pp. 954-955.
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Hayashida T., Yamaguchi Y., Kirchner K., Nagashima H. Isolable Yet Highly Reactive Cationic Organoruthenium(II) Amidinates, [Ru(η6-C6R6)(η-amidinate)]+X−, Showing Signs of Coordinative Unsaturation: Isoelectronic Complexes of Ru(η5-C5Me5)(η-amidinate) // Chemistry Letters. 2001. Vol. 30. No. 10. pp. 954-955.
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TY - JOUR
DO - 10.1246/cl.2001.954
UR - https://doi.org/10.1246/cl.2001.954
TI - Isolable Yet Highly Reactive Cationic Organoruthenium(II) Amidinates, [Ru(η6-C6R6)(η-amidinate)]+X−, Showing Signs of Coordinative Unsaturation: Isoelectronic Complexes of Ru(η5-C5Me5)(η-amidinate)
T2 - Chemistry Letters
AU - Hayashida, Taizo
AU - Yamaguchi, Yoshitaka
AU - Kirchner, Karl
AU - Nagashima, Hideo
PY - 2001
DA - 2001/10/01
PB - Oxford University Press
SP - 954-955
IS - 10
VL - 30
SN - 0366-7022
SN - 1348-0715
ER -
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BibTex (up to 50 authors)
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@article{2001_Hayashida,
author = {Taizo Hayashida and Yoshitaka Yamaguchi and Karl Kirchner and Hideo Nagashima},
title = {Isolable Yet Highly Reactive Cationic Organoruthenium(II) Amidinates, [Ru(η6-C6R6)(η-amidinate)]+X−, Showing Signs of Coordinative Unsaturation: Isoelectronic Complexes of Ru(η5-C5Me5)(η-amidinate)},
journal = {Chemistry Letters},
year = {2001},
volume = {30},
publisher = {Oxford University Press},
month = {oct},
url = {https://doi.org/10.1246/cl.2001.954},
number = {10},
pages = {954--955},
doi = {10.1246/cl.2001.954}
}
Cite this
MLA
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Hayashida, Taizo, et al. “Isolable Yet Highly Reactive Cationic Organoruthenium(II) Amidinates, [Ru(η6-C6R6)(η-amidinate)]+X−, Showing Signs of Coordinative Unsaturation: Isoelectronic Complexes of Ru(η5-C5Me5)(η-amidinate).” Chemistry Letters, vol. 30, no. 10, Oct. 2001, pp. 954-955. https://doi.org/10.1246/cl.2001.954.