Radiochimica Acta

, том 103 , издание 3 , страницы 175-185

Partitioning and speciation of Pu in the sedimentary rocks aquifer from the deep liquid nuclear waste disposal

Тип публикации: Journal Article

Дата публикации: 2014-12-18

De Gruyter Brill

Radiochimica Acta

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SJR: 0.268

CiteScore: 3

Impact factor: 1.7

ISSN: 00338230, 21933405

DOI: 10.1515/RACT-2014-2344

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Physical and Theoretical Chemistry

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Plutonium partitioning and speciation was studied under the conditions of a liquid nuclear waste repository site. The dominating effect of corrosion products (Fe and Cr) oxides on plutonium partitioning was established in batch sorption tests at 150 ℃ and by using sequential extraction. Various techniques including Mössbauer spectrometry, XRD and TEM were used to characterize Fe/Cr oxide phases that form both precipitates and surface coatings which sorb plutonium. The sorption and speciation of plutonium was modeled thermodynamically using Pourbaix diagram that takes into account both surface complexation reaction and precipitation of insoluble PuO₂.

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Kalmykov S. N. et al. Partitioning and speciation of Pu in the sedimentary rocks aquifer from the deep liquid nuclear waste disposal // Radiochimica Acta. 2014. Vol. 103. No. 3. pp. 175-185.

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Vlasova I. E., Romanchuk A. Yu., Zakharova E. V., Volkova A. G., Presnyakov I. A. Partitioning and speciation of Pu in the sedimentary rocks aquifer from the deep liquid nuclear waste disposal // Radiochimica Acta. 2014. Vol. 103. No. 3. pp. 175-185.

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TY - JOUR

DO - 10.1515/RACT-2014-2344

UR - https://www.degruyter.com/document/doi/10.1515/ract-2014-2344/html

TI - Partitioning and speciation of Pu in the sedimentary rocks aquifer from the deep liquid nuclear waste disposal

T2 - Radiochimica Acta

AU - Vlasova, Irina E

AU - Romanchuk, Anna Yu

AU - Zakharova, Elena V.

AU - Volkova, Anna G

AU - Presnyakov, Igor A.

PY - 2014

DA - 2014/12/18

PB - De Gruyter Brill

SP - 175-185

IS - 3

VL - 103

SN - 0033-8230

SN - 2193-3405

ER -

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@article{2014_Kalmykov,

author = {Irina E Vlasova and Anna Yu Romanchuk and Elena V. Zakharova and Anna G Volkova and Igor A. Presnyakov},

title = {Partitioning and speciation of Pu in the sedimentary rocks aquifer from the deep liquid nuclear waste disposal},

journal = {Radiochimica Acta},

year = {2014},

volume = {103},

publisher = {De Gruyter Brill},

month = {dec},

url = {https://www.degruyter.com/document/doi/10.1515/ract-2014-2344/html},

number = {3},

pages = {175--185},

doi = {10.1515/RACT-2014-2344}

}

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Kalmykov, Stepan N., et al. “Partitioning and speciation of Pu in the sedimentary rocks aquifer from the deep liquid nuclear waste disposal.” Radiochimica Acta, vol. 103, no. 3, Dec. 2014, pp. 175-185. https://www.degruyter.com/document/doi/10.1515/ract-2014-2344/html.