Photoreduction of Pu(V,VI) by TiO2
Stepan N. Kalmykov
1, 2, 3
,
Alexander V Egorov
1
,
Yan V. Zubavichus
3
,
Andrei A. Shiryaev
1, 4
,
Eugene A Smirnov
1
,
Alexey V. Garshev
1
Publication type: Journal Article
Publication date: 2016-08-25
scimago Q4
wos Q2
SJR: 0.268
CiteScore: 3.0
Impact factor: 1.7
ISSN: 00338230, 21933405
Physical and Theoretical Chemistry
Abstract
In this study, the effect of light on the kinetics and speciation of plutonium at its interaction with particles of TiO2 under different light conditions is shown for the first time. It was found that sorption was followed by reduction of the plutonium to Pu(IV). In this, the reduction reaction and sorption in conditions of the presence of light proceed significantly more rapidly due to the photocatalytic activity of titanium dioxide, providing a source of electrons for the reaction. Spectral methods (XAFS and TEM) showed that plutonium forms nanoclusters with the structure of PuO2, which decorate the surface of the solid phase.
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Total citations:
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Citations from 2024:
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GOST
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Romanchuk A. Yu. et al. Photoreduction of Pu(V,VI) by TiO2 // Radiochimica Acta. 2016. Vol. 104. No. 12. pp. 843-851.
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Romanchuk A. Yu., Kalmykov S. N., Egorov A. V., Zubavichus Y. V., Shiryaev A. A., Smirnov E. A., Garshev A. V. Photoreduction of Pu(V,VI) by TiO2 // Radiochimica Acta. 2016. Vol. 104. No. 12. pp. 843-851.
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RIS
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TY - JOUR
DO - 10.1515/RACT-2015-2494
UR - https://www.degruyter.com/document/doi/10.1515/ract-2015-2494/html
TI - Photoreduction of Pu(V,VI) by TiO2
T2 - Radiochimica Acta
AU - Romanchuk, Anna Yu
AU - Kalmykov, Stepan N.
AU - Egorov, Alexander V
AU - Zubavichus, Yan V.
AU - Shiryaev, Andrei A.
AU - Smirnov, Eugene A
AU - Garshev, Alexey V.
PY - 2016
DA - 2016/08/25
PB - Walter de Gruyter
SP - 843-851
IS - 12
VL - 104
SN - 0033-8230
SN - 2193-3405
ER -
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BibTex (up to 50 authors)
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@article{2016_Romanchuk,
author = {Anna Yu Romanchuk and Stepan N. Kalmykov and Alexander V Egorov and Yan V. Zubavichus and Andrei A. Shiryaev and Eugene A Smirnov and Alexey V. Garshev},
title = {Photoreduction of Pu(V,VI) by TiO2},
journal = {Radiochimica Acta},
year = {2016},
volume = {104},
publisher = {Walter de Gruyter},
month = {aug},
url = {https://www.degruyter.com/document/doi/10.1515/ract-2015-2494/html},
number = {12},
pages = {843--851},
doi = {10.1515/RACT-2015-2494}
}
Cite this
MLA
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Romanchuk, Anna Yu., et al. “Photoreduction of Pu(V,VI) by TiO2.” Radiochimica Acta, vol. 104, no. 12, Aug. 2016, pp. 843-851. https://www.degruyter.com/document/doi/10.1515/ract-2015-2494/html.