Zeitschrift fur Naturforschung - Section B Journal of Chemical Sciences, volume 53, issue 1, pages 63-74
Unusual Bonding in Ternary Nitrides: Preparation, Structure and Properties of Ce2MnN3.
2
University of Missouri Research Reactor, Columbia, MO 65211, USA
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Publication type: Journal Article
Publication date: 1998-01-01
Quartile SCImago
Q3
Quartile WOS
Q4
Impact factor: 0.8
ISSN: 09320776
General Chemistry
Abstract
Ce2MnN3 was prepared by reaction of cerium nitride and manganese with nitrogen gas at 900 °C. It crystallizes isotypic to AC2MN3 (Ac = U, Th; M = Cr, Mn) and Ce2CrN3, space group Immm (No. 71), a = 3.74994(6) Å, b = 3.44450(6) Å and c = 12.4601(2) Å. The manganese atoms are coordinated in a nearly square planar fashion by four nitrogen atoms. These corner-connected MnN4 units form infinite 1 ∞[MnN2N2/2] chains, which run parallel to each other along the crystallographic a-axis, forming the motif of hexagonal rod packing. Cerium atoms connect the chains into a three-dimensional network. The results of measurements of the magnetic susceptibility, as well as of the electrical resistivity suggest metallic behavior. Electronic effects leading to shorter bonds between manganese and bridging nitrogen atoms than between manganese and terminal nitrogen atoms in the 1 ∞[MnN2N2/2] chains were investigated through extended Hückel and LMTO band structure calculations. Issues pertaining to stability of this and some other nitridometallate structures are discussed.
Top-30
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1 publication, 3.23%
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1 publication, 3.23%
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1 publication, 3.23%
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Citations by publishers
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2
4
6
8
10
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Wiley
10 publications, 32.26%
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Elsevier
8 publications, 25.81%
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3 publications, 9.68%
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2 publications, 6.45%
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1 publication, 3.23%
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Royal Society of Chemistry (RSC)
1 publication, 3.23%
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1 publication, 3.23%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 3.23%
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2
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10
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Niewa R. et al. Unusual Bonding in Ternary Nitrides: Preparation, Structure and Properties of Ce2MnN3. // Zeitschrift fur Naturforschung - Section B Journal of Chemical Sciences. 1998. Vol. 53. No. 1. pp. 63-74.
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Niewa R., Vajenine G. V., DiSalvo F. J., Luob H., Yelon W. B. Unusual Bonding in Ternary Nitrides: Preparation, Structure and Properties of Ce2MnN3. // Zeitschrift fur Naturforschung - Section B Journal of Chemical Sciences. 1998. Vol. 53. No. 1. pp. 63-74.
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TY - JOUR
DO - 10.1515/znb-1998-0113
UR - https://doi.org/10.1515/znb-1998-0113
TI - Unusual Bonding in Ternary Nitrides: Preparation, Structure and Properties of Ce2MnN3.
T2 - Zeitschrift fur Naturforschung - Section B Journal of Chemical Sciences
AU - Niewa, Rainer
AU - Vajenine, Grigori V.
AU - DiSalvo, Francis J.
AU - Luob, Haihua
AU - Yelon, William B.
PY - 1998
DA - 1998/01/01 00:00:00
PB - Walter de Gruyter
SP - 63-74
IS - 1
VL - 53
SN - 0932-0776
ER -
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@article{1998_Niewa,
author = {Rainer Niewa and Grigori V. Vajenine and Francis J. DiSalvo and Haihua Luob and William B. Yelon},
title = {Unusual Bonding in Ternary Nitrides: Preparation, Structure and Properties of Ce2MnN3.},
journal = {Zeitschrift fur Naturforschung - Section B Journal of Chemical Sciences},
year = {1998},
volume = {53},
publisher = {Walter de Gruyter},
month = {jan},
url = {https://doi.org/10.1515/znb-1998-0113},
number = {1},
pages = {63--74},
doi = {10.1515/znb-1998-0113}
}
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MLA
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Niewa, Rainer, et al. “Unusual Bonding in Ternary Nitrides: Preparation, Structure and Properties of Ce2MnN3..” Zeitschrift fur Naturforschung - Section B Journal of Chemical Sciences, vol. 53, no. 1, Jan. 1998, pp. 63-74. https://doi.org/10.1515/znb-1998-0113.