Open Access
A Panchromatic Cyclometalated Iridium Dye Based on 2-Thienyl-Perimidine
Paulina Kalle
1
,
Marina A. Kiseleva
1, 2
,
Sergei V. Tatarin
1, 2
,
Daniil E. Smirnov
1, 2
,
Viktor V Emets
3
,
2
Publication type: Journal Article
Publication date: 2022-05-17
PubMed ID:
35630677
Organic Chemistry
Drug Discovery
Physical and Theoretical Chemistry
Pharmaceutical Science
Molecular Medicine
Analytical Chemistry
Chemistry (miscellaneous)
Abstract
Though 2-arylperimidines have never been used in iridium(III) chemistry, the present study on structural, electronic and optical properties of N-unsubstituted and N-methylated 2-(2-thienyl)perimidines, supported by DFT/TDDFT calculations, has shown that these ligands are promising candidates for construction of light-harvesting iridium(III) complexes. In contrast to N-H perimidine, the N-methylated ligand gave the expected cyclometalated μ-chloro-bridged iridium(III) dimer which was readily converted to a cationic heteroleptic complex with 4,4′-dicarboxy-2,2′-bipyridine. The resulting iridium(III) dye exhibited panchromatic absorption up to 1000 nm and was tested in a dye-sensitized solar cell.
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15
Total citations:
15
Citations from 2024:
6
(42.86%)
The most citing journal
Citations in journal:
2
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MLA
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GOST
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Kalle P. et al. A Panchromatic Cyclometalated Iridium Dye Based on 2-Thienyl-Perimidine // Molecules. 2022. Vol. 27. No. 10. p. 3201.
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Kalle P., Kiseleva M. A., Tatarin S. V., Smirnov D. E., Zakharov A. Y., Emets V. V., Churakov A. V., Bezzubov S. I. A Panchromatic Cyclometalated Iridium Dye Based on 2-Thienyl-Perimidine // Molecules. 2022. Vol. 27. No. 10. p. 3201.
Cite this
RIS
Copy
TY - JOUR
DO - 10.3390/molecules27103201
UR - https://www.mdpi.com/1420-3049/27/10/3201
TI - A Panchromatic Cyclometalated Iridium Dye Based on 2-Thienyl-Perimidine
T2 - Molecules
AU - Kalle, Paulina
AU - Kiseleva, Marina A.
AU - Tatarin, Sergei V.
AU - Smirnov, Daniil E.
AU - Zakharov, Alexander Y
AU - Emets, Viktor V
AU - Churakov, Andrei V.
AU - Bezzubov, Stanislav I.
PY - 2022
DA - 2022/05/17
PB - MDPI
SP - 3201
IS - 10
VL - 27
PMID - 35630677
SN - 1420-3049
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2022_Kalle,
author = {Paulina Kalle and Marina A. Kiseleva and Sergei V. Tatarin and Daniil E. Smirnov and Alexander Y Zakharov and Viktor V Emets and Andrei V. Churakov and Stanislav I. Bezzubov},
title = {A Panchromatic Cyclometalated Iridium Dye Based on 2-Thienyl-Perimidine},
journal = {Molecules},
year = {2022},
volume = {27},
publisher = {MDPI},
month = {may},
url = {https://www.mdpi.com/1420-3049/27/10/3201},
number = {10},
pages = {3201},
doi = {10.3390/molecules27103201}
}
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MLA
Copy
Kalle, Paulina, et al. “A Panchromatic Cyclometalated Iridium Dye Based on 2-Thienyl-Perimidine.” Molecules, vol. 27, no. 10, May. 2022, p. 3201. https://www.mdpi.com/1420-3049/27/10/3201.