Open Access
Applied Sciences (Switzerland), volume 10, issue 12, pages 4185
Recent Advances in Lithiophilic Porous Framework toward Dendrite-Free Lithium Metal Anode
1
Department of Electrical Engineering and Computer Science, South Dakota State University, Brookings, SD 57007, USA
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Publication type: Journal Article
Publication date: 2020-06-18
Journal:
Applied Sciences (Switzerland)
Quartile SCImago
Q2
Quartile WOS
Q2
Impact factor: 2.7
ISSN: 20763417
Computer Science Applications
Process Chemistry and Technology
General Materials Science
Instrumentation
General Engineering
Fluid Flow and Transfer Processes
Abstract
Rechargeable lithium metal anode (LMA) based batteries have attracted great attention as next-generation high-energy-density storage systems to fuel the extensive practical applications in portable electronics and electric vehicles. However, the formation of unstable solid-electrolyte- interphase (SEI) and growth of lithium dendrite during plating/stripping cycles stimulate safety concern, poor coulombic efficiency (CE), and short lifespan of the lithium metal batteries (LMBs). To address these issues, the rational design of micro/nanostructured Li hosts are widely adopted in LMBs. The high surface area of the interconnected conductive framework can homogenize the Li-ion flux distribution, lower the effective current density, and provides sufficient space for Li accommodation. However, the poor lithiophilicity of the micro/nanostructure host cannot govern the initial lithium nucleation, which leads to the non-uniform/dendritic Li deposition and unstable SEI formation. As a result, the nucleation overpotential and voltage hysteresis increases, which eventually leads to poor battery cycling performance. Thus, it is imperative to decorate a micro/nanostructured Li host with lithiophilic coatings or seeds for serving as a homogeneous nucleation site to guide the uniform lithium deposition. In this review, we summarize research progress on porous metal and non-metal based lithiophilic micro/nanostructured Li hosts. We present the synthesis, structural properties, and the significance of lithiophilic decorated micro/nanostructured Li host in the LMBs. Finally, the perspectives and critical challenges needed to address for the further improvement of LMBs are concluded.
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1 publication, 2.5%
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2
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Pathak R., Zhou Y., Qiao Q. Recent Advances in Lithiophilic Porous Framework toward Dendrite-Free Lithium Metal Anode // Applied Sciences (Switzerland). 2020. Vol. 10. No. 12. p. 4185.
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Pathak R., Zhou Y., Qiao Q. Recent Advances in Lithiophilic Porous Framework toward Dendrite-Free Lithium Metal Anode // Applied Sciences (Switzerland). 2020. Vol. 10. No. 12. p. 4185.
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TY - JOUR
DO - 10.3390/app10124185
UR - https://doi.org/10.3390/app10124185
TI - Recent Advances in Lithiophilic Porous Framework toward Dendrite-Free Lithium Metal Anode
T2 - Applied Sciences (Switzerland)
AU - Zhou, Yue
AU - Qiao, Qiquan
AU - Pathak, Rajesh
PY - 2020
DA - 2020/06/18 00:00:00
PB - Multidisciplinary Digital Publishing Institute (MDPI)
SP - 4185
IS - 12
VL - 10
SN - 2076-3417
ER -
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@article{2020_Pathak,
author = {Yue Zhou and Qiquan Qiao and Rajesh Pathak},
title = {Recent Advances in Lithiophilic Porous Framework toward Dendrite-Free Lithium Metal Anode},
journal = {Applied Sciences (Switzerland)},
year = {2020},
volume = {10},
publisher = {Multidisciplinary Digital Publishing Institute (MDPI)},
month = {jun},
url = {https://doi.org/10.3390/app10124185},
number = {12},
pages = {4185},
doi = {10.3390/app10124185}
}
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MLA
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Pathak, Rajesh, et al. “Recent Advances in Lithiophilic Porous Framework toward Dendrite-Free Lithium Metal Anode.” Applied Sciences (Switzerland), vol. 10, no. 12, Jun. 2020, p. 4185. https://doi.org/10.3390/app10124185.