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An investigation into the bulk and surface phase transformations of bimetallic Pd-In/Al2 O3 catalyst during reductive and oxidative treatments in situ
2
Publication type: Journal Article
Publication date: 2021-07-18
Catalysis
Physical and Theoretical Chemistry
Abstract
A series of oxidative treatments of PdIn-supported intermetallic nanoparticles at different temperatures were performed. The bulk and surface structure of catalyst during phase transformation was investigated by bulk- and surface-sensitive techniques (in situ XAFS, DRIFTS of adsorbed CO). It was found that comparison of palladium and indium fractions in bulk and on the surface suggests the formation of a «core-shell» structure. According to obtained results, the core consists of In-depleted intermetallic compound or inhomogeneous bimetallic phase with the inner core of metallic Pd, when a mixture of indium oxide, metallic palladium and small part of PdIn is present on the surface.
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7
Total citations:
7
Citations from 2024:
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(57%)
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Smirnova N. S. et al. An investigation into the bulk and surface phase transformations of bimetallic Pd-In/Al2O3 catalyst during reductive and oxidative treatments in situ // Catalysts. 2021. Vol. 11. No. 7. p. 859.
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Smirnova N. S., Khramov E. V., Baeva G. N., Markov P. V., Bukhtiyarov A. V., Zubavichus Y. V., Stakheev A. Yu. An investigation into the bulk and surface phase transformations of bimetallic Pd-In/Al2O3 catalyst during reductive and oxidative treatments in situ // Catalysts. 2021. Vol. 11. No. 7. p. 859.
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TY - JOUR
DO - 10.3390/catal11070859
UR - https://doi.org/10.3390/catal11070859
TI - An investigation into the bulk and surface phase transformations of bimetallic Pd-In/Al2O3 catalyst during reductive and oxidative treatments in situ
T2 - Catalysts
AU - Smirnova, Nadezhda S
AU - Khramov, Evgeny V
AU - Baeva, Galina N
AU - Markov, Pavel V
AU - Bukhtiyarov, Andrey V
AU - Zubavichus, Yan V.
AU - Stakheev, Alexander Yu
PY - 2021
DA - 2021/07/18
PB - MDPI
SP - 859
IS - 7
VL - 11
SN - 2073-4344
ER -
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@article{2021_Smirnova,
author = {Nadezhda S Smirnova and Evgeny V Khramov and Galina N Baeva and Pavel V Markov and Andrey V Bukhtiyarov and Yan V. Zubavichus and Alexander Yu Stakheev},
title = {An investigation into the bulk and surface phase transformations of bimetallic Pd-In/Al2O3 catalyst during reductive and oxidative treatments in situ},
journal = {Catalysts},
year = {2021},
volume = {11},
publisher = {MDPI},
month = {jul},
url = {https://doi.org/10.3390/catal11070859},
number = {7},
pages = {859},
doi = {10.3390/catal11070859}
}
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MLA
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Smirnova, Nadezhda S., et al. “An investigation into the bulk and surface phase transformations of bimetallic Pd-In/Al2O3 catalyst during reductive and oxidative treatments in situ.” Catalysts, vol. 11, no. 7, Jul. 2021, p. 859. https://doi.org/10.3390/catal11070859.