Open Access
Reductive Transformation of O-, N-, S-Containing Aromatic Compounds under Hydrogen Transfer Conditions: Effect of the Process on the Ni-Based Catalyst
Publication type: Journal Article
Publication date: 2023-10-12
PubMed ID:
37894520
Organic Chemistry
Drug Discovery
Physical and Theoretical Chemistry
Pharmaceutical Science
Molecular Medicine
Analytical Chemistry
Chemistry (miscellaneous)
Abstract
The influence of the reaction medium on the surface structure and properties of a Ni-based catalyst used for the reductive transformations of O-, N-, and S-containing aromatic substrates under hydrogen transfer conditions has been studied. The catalysts were characterized by XRD, XPS, and IR spectroscopy and TEM methods before and after the reductive reaction. It has been shown that the conversion of 1-benzothiophene causes irreversible poisoning of the catalyst surface with the formation of the Ni2S3 phase, whereas the conversion of naphthalene, 1-benzofuran, and indole does not cause any phase change of the catalyst at 250 °C. However, after the indole conversion, the catalyst surface remains enriched with N-containing compounds, which are evenly distributed over the surface.
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Total citations:
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Citations from 2025:
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(83.34%)
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Nesterov N. S. et al. Reductive Transformation of O-, N-, S-Containing Aromatic Compounds under Hydrogen Transfer Conditions: Effect of the Process on the Ni-Based Catalyst // Molecules. 2023. Vol. 28. No. 20. p. 7041.
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Nesterov N. S., Pakharukova V. P., Philippov A. A., Prosvirin I. P., Shalygin A. S., Martyanov O. N. Reductive Transformation of O-, N-, S-Containing Aromatic Compounds under Hydrogen Transfer Conditions: Effect of the Process on the Ni-Based Catalyst // Molecules. 2023. Vol. 28. No. 20. p. 7041.
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RIS
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TY - JOUR
DO - 10.3390/molecules28207041
UR - https://www.mdpi.com/1420-3049/28/20/7041
TI - Reductive Transformation of O-, N-, S-Containing Aromatic Compounds under Hydrogen Transfer Conditions: Effect of the Process on the Ni-Based Catalyst
T2 - Molecules
AU - Nesterov, Nikolai S
AU - Pakharukova, Vera P.
AU - Philippov, A A
AU - Prosvirin, Igor P.
AU - Shalygin, Anton S.
AU - Martyanov, Oleg N
PY - 2023
DA - 2023/10/12
PB - MDPI
SP - 7041
IS - 20
VL - 28
PMID - 37894520
SN - 1420-3049
ER -
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BibTex (up to 50 authors)
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@article{2023_Nesterov,
author = {Nikolai S Nesterov and Vera P. Pakharukova and A A Philippov and Igor P. Prosvirin and Anton S. Shalygin and Oleg N Martyanov},
title = {Reductive Transformation of O-, N-, S-Containing Aromatic Compounds under Hydrogen Transfer Conditions: Effect of the Process on the Ni-Based Catalyst},
journal = {Molecules},
year = {2023},
volume = {28},
publisher = {MDPI},
month = {oct},
url = {https://www.mdpi.com/1420-3049/28/20/7041},
number = {20},
pages = {7041},
doi = {10.3390/molecules28207041}
}
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MLA
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Nesterov, Nikolai S., et al. “Reductive Transformation of O-, N-, S-Containing Aromatic Compounds under Hydrogen Transfer Conditions: Effect of the Process on the Ni-Based Catalyst.” Molecules, vol. 28, no. 20, Oct. 2023, p. 7041. https://www.mdpi.com/1420-3049/28/20/7041.