Open Access
Nanomaterials, volume 10, issue 11, pages 2183
Atomic Layer Deposition of Mixed-Layered Aurivillius Phase on TiO2 Nanotubes: Synthesis, Characterization and Photoelectrocatalytic Properties
Orudzhev Farid
1
,
Sobola Dinara
1, 2, 3
,
Isaev Abdulgalim
1
,
Wang Chuanyi
4
,
Kadiev Makhmud
1
,
Kaviyarasu Kasinathan
5, 6
2
Department of Physics, Faculty of Electrical Engineering and Communication, Brno University of Technology, Technická 2848/8, 61600 Brno, Czech Republic
|
3
Central European Institute of Technology BUT, Purkyňova 123, 61200 Brno, Czech Republic
|
5
UNESCO-UNISA Africa Chair in Nanoscience’s/Nanotechnology Laboratories, College of Graduate Studies, University of South Africa (UNISA), Muckleneuk Ridge, P.O. Box 392, Pretoria 0003, South Africa
|
6
Nanosciences African Network (NANOAFNET), Materials Research Group (MRG), iThemba LABS-National Research Foundation (NRF), 1 Old Faure Road, 7129, P.O. Box 722, Somerset West 8000, South Africa
|
Publication type: Journal Article
Publication date: 2020-11-02
PubMed ID:
33147745
General Chemical Engineering
General Materials Science
Abstract
For the first time, one-dimensional phase-modulated structures consisting of two different layered Aurivillius phases with alternating five and six perovskite-like layers were obtained by atomic layer deposition (ALD) on the surface of TiO2 nanotubes (Nt). It was shown that the use of vertically oriented TiO2 Nt as the substrate and the ALD technology of a two-layer Bi2O3-FeOx sandwich-structure make it possible to obtain a layered structure due to self-organization during annealing. A detailed study by scanning electron microscopy (SEM) and transmission electron microscopy (TEM) showed that the coating is conformal. Raman spectroscopic analysis indicated the structure of the layered Aurivillius phases. Transient photocurrent responses under Ultraviolet–Visible (UV-Vis) light irradiation show that the ALD coating benefits the efficiency of photon excitation of electrons. The results of the photoelectrocatalytic experiments (PEC) with methyl orange degradation as a model demonstrate the significant potential of the synthesized structure as a photocatalyst. Photoluminescent measurement showed a decrease in the probability of recombination of photogenerated electron–hole pairs for ALD-coated TiO2 Nt, which demonstrates the high potential of these structures for use in photocatalytic and photoelectrochemical applications.
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Citations by publishers
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1 publication, 3.03%
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2
4
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14
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- We do not take into account publications that without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Orudzhev F. et al. Atomic Layer Deposition of Mixed-Layered Aurivillius Phase on TiO2 Nanotubes: Synthesis, Characterization and Photoelectrocatalytic Properties // Nanomaterials. 2020. Vol. 10. No. 11. p. 2183.
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Orudzhev F., Ramazanov S., Sobola D., Isaev A., Wang C., Magomedova A., Kadiev M., Kaviyarasu K. Atomic Layer Deposition of Mixed-Layered Aurivillius Phase on TiO2 Nanotubes: Synthesis, Characterization and Photoelectrocatalytic Properties // Nanomaterials. 2020. Vol. 10. No. 11. p. 2183.
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TY - JOUR
DO - 10.3390/nano10112183
UR - https://doi.org/10.3390%2Fnano10112183
TI - Atomic Layer Deposition of Mixed-Layered Aurivillius Phase on TiO2 Nanotubes: Synthesis, Characterization and Photoelectrocatalytic Properties
T2 - Nanomaterials
AU - Isaev, Abdulgalim
AU - Kadiev, Makhmud
AU - Magomedova, Asiyat
AU - Kaviyarasu, Kasinathan
AU - Orudzhev, Farid
AU - Ramazanov, Shikhgasan
AU - Sobola, Dinara
AU - Wang, Chuanyi
PY - 2020
DA - 2020/11/02 00:00:00
PB - Multidisciplinary Digital Publishing Institute (MDPI)
SP - 2183
IS - 11
VL - 10
PMID - 33147745
SN - 2079-4991
ER -
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@article{2020_Orudzhev,
author = {Abdulgalim Isaev and Makhmud Kadiev and Asiyat Magomedova and Kasinathan Kaviyarasu and Farid Orudzhev and Shikhgasan Ramazanov and Dinara Sobola and Chuanyi Wang},
title = {Atomic Layer Deposition of Mixed-Layered Aurivillius Phase on TiO2 Nanotubes: Synthesis, Characterization and Photoelectrocatalytic Properties},
journal = {Nanomaterials},
year = {2020},
volume = {10},
publisher = {Multidisciplinary Digital Publishing Institute (MDPI)},
month = {nov},
url = {https://doi.org/10.3390%2Fnano10112183},
number = {11},
pages = {2183},
doi = {10.3390/nano10112183}
}
Cite this
MLA
Copy
Orudzhev, Farid, et al. “Atomic Layer Deposition of Mixed-Layered Aurivillius Phase on TiO2 Nanotubes: Synthesis, Characterization and Photoelectrocatalytic Properties.” Nanomaterials, vol. 10, no. 11, Nov. 2020, p. 2183. https://doi.org/10.3390%2Fnano10112183.