Rational Construction of Chiral Octanuclear Metallacycles Consisting of Octahedral CoIII, Square-Planar PdII, and Linear AuI or AgI Ions
Takumi Konno
1
,
Yu Chikamoto
2
,
Ken-ichi Okamoto
3
,
Tadashi Yamaguchi
4
,
TASUKU ITO
4
,
Masakazu Hirotsu
2
1
Publication type: Journal Article
Publication date: 2000-11-17
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
General Chemistry
Catalysis
Abstract
Octahedral fac(S)-[CoIII(aet)3] molecules (aet=NH2CH2CH2S−) react with square-planar PdII ions to form a sulfur-bridged CoPdII trinuclear complex [Pd{Co(aet)3}2]2+, accompanied by the geometrical isomerization from fac(S) to mer(S). This complex was found to act as a sulfur-donating trinuclear-metalloligand toward linear AuI and AgI ions to afford CoPdM metallacycles with 16 chiral centers, [M{PdII[CoIII(aet)3]2}2]6+ (M=Ag, Au (1)), which were successfully resolved into the (Δ)4(R)12 and (Λ)4(S)12 enantiomers.
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Konno T. et al. Rational Construction of Chiral Octanuclear Metallacycles Consisting of Octahedral CoIII, Square-Planar PdII, and Linear AuI or AgI Ions // Angewandte Chemie - International Edition. 2000. Vol. 39. No. 22. pp. 4098-4101.
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Konno T., Chikamoto Yu., Okamoto K., Yamaguchi T., ITO T., Hirotsu M. Rational Construction of Chiral Octanuclear Metallacycles Consisting of Octahedral CoIII, Square-Planar PdII, and Linear AuI or AgI Ions // Angewandte Chemie - International Edition. 2000. Vol. 39. No. 22. pp. 4098-4101.
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TY - JOUR
DO - 10.1002/1521-3773(20001117)39:22<4098::aid-anie4098>3.0.co;2-y
UR - https://onlinelibrary.wiley.com/doi/10.1002/1521-3773(20001117)39:22<4098::AID-ANIE4098>3.0.CO;2-Y
TI - Rational Construction of Chiral Octanuclear Metallacycles Consisting of Octahedral CoIII, Square-Planar PdII, and Linear AuI or AgI Ions
T2 - Angewandte Chemie - International Edition
AU - Konno, Takumi
AU - Chikamoto, Yu
AU - Okamoto, Ken-ichi
AU - Yamaguchi, Tadashi
AU - ITO, TASUKU
AU - Hirotsu, Masakazu
PY - 2000
DA - 2000/11/17
PB - Wiley
SP - 4098-4101
IS - 22
VL - 39
PMID - 11093218
SN - 1433-7851
SN - 1521-3773
ER -
Cite this
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@article{2000_Konno,
author = {Takumi Konno and Yu Chikamoto and Ken-ichi Okamoto and Tadashi Yamaguchi and TASUKU ITO and Masakazu Hirotsu},
title = {Rational Construction of Chiral Octanuclear Metallacycles Consisting of Octahedral CoIII, Square-Planar PdII, and Linear AuI or AgI Ions},
journal = {Angewandte Chemie - International Edition},
year = {2000},
volume = {39},
publisher = {Wiley},
month = {nov},
url = {https://onlinelibrary.wiley.com/doi/10.1002/1521-3773(20001117)39:22<4098::AID-ANIE4098>3.0.CO;2-Y},
number = {22},
pages = {4098--4101},
doi = {10.1002/1521-3773(20001117)39:22<4098::aid-anie4098>3.0.co;2-y}
}
Cite this
MLA
Copy
Konno, Takumi, et al. “Rational Construction of Chiral Octanuclear Metallacycles Consisting of Octahedral CoIII, Square-Planar PdII, and Linear AuI or AgI Ions.” Angewandte Chemie - International Edition, vol. 39, no. 22, Nov. 2000, pp. 4098-4101. https://onlinelibrary.wiley.com/doi/10.1002/1521-3773(20001117)39:22<4098::AID-ANIE4098>3.0.CO;2-Y.