Palladium-Catalyzed Methoxycarbonylation of 1,3-Butadiene: Catalysis and Mechanistic Studies
Publication type: Journal Article
Publication date: 2002-07-01
scimago Q1
wos Q1
SJR: 0.930
CiteScore: 8.0
Impact factor: 4.0
ISSN: 16154150, 16154169
General Chemistry
Abstract
The palladium-catalyzed methoxycarbonylation of 1,3-butadiene to methyl 3-pentenoate has been studied. Intermediates of the proposed catalytic cycle were synthesized and the elementary steps of the reaction have been investigated in detail. It is shown that the first step of the catalytic cycle, the formation of crotylpalladium complexes from 1,3-butadiene, proceeds even at room temperature. Examination of the influence of different reaction parameters on product yield and selectivity demonstrate the importance of chelating phosphine ligands and benzoic acids as additive in order to get good results.
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39
Total citations:
39
Citations from 2024:
3
(7%)
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GOST
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Beller M., Krotz A., Baumann W. Palladium-Catalyzed Methoxycarbonylation of 1,3-Butadiene: Catalysis and Mechanistic Studies // Advanced Synthesis and Catalysis. 2002. Vol. 344. No. 5. p. 517.
GOST all authors (up to 50)
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Beller M., Krotz A., Baumann W. Palladium-Catalyzed Methoxycarbonylation of 1,3-Butadiene: Catalysis and Mechanistic Studies // Advanced Synthesis and Catalysis. 2002. Vol. 344. No. 5. p. 517.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1002/1615-4169(200207)344:5<517::aid-adsc517>3.0.co;2-q
UR - https://doi.org/10.1002/1615-4169(200207)344:5<517::aid-adsc517>3.0.co;2-q
TI - Palladium-Catalyzed Methoxycarbonylation of 1,3-Butadiene: Catalysis and Mechanistic Studies
T2 - Advanced Synthesis and Catalysis
AU - Beller, Matthias
AU - Krotz, Andreas
AU - Baumann, Wolfgang
PY - 2002
DA - 2002/07/01
PB - Wiley
SP - 517
IS - 5
VL - 344
SN - 1615-4150
SN - 1615-4169
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2002_Beller,
author = {Matthias Beller and Andreas Krotz and Wolfgang Baumann},
title = {Palladium-Catalyzed Methoxycarbonylation of 1,3-Butadiene: Catalysis and Mechanistic Studies},
journal = {Advanced Synthesis and Catalysis},
year = {2002},
volume = {344},
publisher = {Wiley},
month = {jul},
url = {https://doi.org/10.1002/1615-4169(200207)344:5<517::aid-adsc517>3.0.co;2-q},
number = {5},
pages = {517},
doi = {10.1002/1615-4169(200207)344:5<517::aid-adsc517>3.0.co;2-q}
}
Cite this
MLA
Copy
Beller, Matthias, et al. “Palladium-Catalyzed Methoxycarbonylation of 1,3-Butadiene: Catalysis and Mechanistic Studies.” Advanced Synthesis and Catalysis, vol. 344, no. 5, Jul. 2002, p. 517. https://doi.org/10.1002/1615-4169(200207)344:5<517::aid-adsc517>3.0.co;2-q.