Advanced Materials, volume 34, issue 10, pages 2102354
High Photocatalytic Oxygen Evolution via Strong Built‐In Electric Field Induced by High Crystallinity of Perylene Imide Supramolecule
2
CTBT Beijing National Data Centre and Beijing Radionuclide Laboratory Beijing 100085 P. R. China
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Publication type: Journal Article
Publication date: 2022-01-31
Journal:
Advanced Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 29.4
ISSN: 09359648, 15214095
General Materials Science
Mechanical Engineering
Mechanics of Materials
Abstract
A highly crystalline perylene imide supramolecular photocatalyst (PDI-NH) is synthesized via imidazole solvent method. The catalyst shows a breakthrough oxygen evolution rate (40.6 mmol g-1 h-1 ) with apparent quantum yield of 10.4% at 400 nm, which is 1353 times higher than the low crystalline PDI-NH. The highly crystalline structure comes from the ordered self-assembly process in molten imidazole solvent via π-π stacking and hydrogen bonding. Further, the excellent performance ascribes to the robust built-in electric field induced by its high crystallinity, which greatly accelerates the charge separation and transfer. What is more, the PDI-NH is quite stable and can be reused over 50 h without performance attenuation. Briefly, the crystalline PDI-NH with strong built-in electric field throws light on photocatalytic oxygen evolution, showing a new perspective for the design of organic photocatalysts.
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1 publication, 1.08%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Sheng Y. et al. High Photocatalytic Oxygen Evolution via Strong Built‐In Electric Field Induced by High Crystallinity of Perylene Imide Supramolecule // Advanced Materials. 2022. Vol. 34. No. 10. p. 2102354.
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Sheng Y., Li W., Xu L., Zhu Y. High Photocatalytic Oxygen Evolution via Strong Built‐In Electric Field Induced by High Crystallinity of Perylene Imide Supramolecule // Advanced Materials. 2022. Vol. 34. No. 10. p. 2102354.
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TY - JOUR
DO - 10.1002/adma.202102354
UR - https://doi.org/10.1002/adma.202102354
TI - High Photocatalytic Oxygen Evolution via Strong Built‐In Electric Field Induced by High Crystallinity of Perylene Imide Supramolecule
T2 - Advanced Materials
AU - Sheng, Yuqiang
AU - Li, Wenlu
AU - Xu, Liangliang
AU - Zhu, Yongfa
PY - 2022
DA - 2022/01/31 00:00:00
PB - Wiley
SP - 2102354
IS - 10
VL - 34
SN - 0935-9648
SN - 1521-4095
ER -
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@article{2022_Sheng,
author = {Yuqiang Sheng and Wenlu Li and Liangliang Xu and Yongfa Zhu},
title = {High Photocatalytic Oxygen Evolution via Strong Built‐In Electric Field Induced by High Crystallinity of Perylene Imide Supramolecule},
journal = {Advanced Materials},
year = {2022},
volume = {34},
publisher = {Wiley},
month = {jan},
url = {https://doi.org/10.1002/adma.202102354},
number = {10},
pages = {2102354},
doi = {10.1002/adma.202102354}
}
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Sheng, Yuqiang, et al. “High Photocatalytic Oxygen Evolution via Strong Built‐In Electric Field Induced by High Crystallinity of Perylene Imide Supramolecule.” Advanced Materials, vol. 34, no. 10, Jan. 2022, p. 2102354. https://doi.org/10.1002/adma.202102354.