Open Access

Advanced Science, volume 3, issue 11, pages 1600180

Transition Metal‐Promoted V ₂ CO ₂ (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction

C. Ling ¹

Li Shi ¹

Yixin Ouyang ¹

Qian Chen ¹

Jinlan Wang ^{1, 2}

Hide authors affiliations Show authors affiliations: 2 affiliations

Department of Physics Southeast University Nanjing 211189 China |

Synergetic Innovation Center for Quantum Effects and Applications (SICQEA) Hunan Normal University Changsha 410081 China |

Publication type: Journal Article

Publication date: 2016-06-28

Wiley

Journal: Advanced Science

Quartile SCImago

Quartile WOS

Impact factor: 15.1

ISSN: 21983844, 21983844

DOI: 10.1002/advs.201600180

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Medicine (miscellaneous)

General Chemical Engineering

General Physics and Astronomy

General Materials Science

General Engineering

Biochemistry, Genetics and Molecular Biology (miscellaneous)

Abstract

Developing alternatives to precious Pt for hydrogen production from water splitting is central to the area of renewable energy. This work predicts extremely high catalytic activity of transition metal (Fe, Co, and Ni) promoted two-dimensional MXenes, fully oxidized vanadium carbides (V2CO2), for hydrogen evolution reaction (HER). The first-principle calculations show that the introduction of transition metal can greatly weaken the strong binding between hydrogen and oxygen and engineer the hydrogen adsorption free energy to the optimal value ≈0 eV by choosing the suitable type and coverage of the promoters as well as the active sites. Strain engineering on the performance of transition metal promoted V2CO2 further reveals that the excellent HER activities can maintain well while those poor ones can be modulated to be highly active. This study provides new possibilities for cost-effective alternatives to Pt in HER and for the application of 2D MXenes.

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Top-30

Citations by journals

	5 10 15 20 25
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 21, 7.22% Journal of Materials Chemistry A 21 publications, 7.22%
Applied Surface Science	Applied Surface Science, 17, 5.84% Applied Surface Science 17 publications, 5.84%
International Journal of Hydrogen Energy	International Journal of Hydrogen Energy, 13, 4.47% International Journal of Hydrogen Energy 13 publications, 4.47%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 10, 3.44% Physical Chemistry Chemical Physics 10 publications, 3.44%
Advanced Materials	Advanced Materials, 8, 2.75% Advanced Materials 8 publications, 2.75%
ACS applied materials & interfaces	ACS applied materials & interfaces, 8, 2.75% ACS applied materials & interfaces 8 publications, 2.75%
Advanced Energy Materials	Advanced Energy Materials, 7, 2.41% Advanced Energy Materials 7 publications, 2.41%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 7, 2.41% Journal of Physical Chemistry C 7 publications, 2.41%
Advanced Functional Materials	Advanced Functional Materials, 6, 2.06% Advanced Functional Materials 6 publications, 2.06%
Chemical Engineering Journal	Chemical Engineering Journal, 6, 2.06% Chemical Engineering Journal 6 publications, 2.06%
Nanoscale	Nanoscale, 6, 2.06% Nanoscale 6 publications, 2.06%
Journal of Catalysis	Journal of Catalysis, 5, 1.72% Journal of Catalysis 5 publications, 1.72%
Chinese Journal of Catalysis	Chinese Journal of Catalysis, 4, 1.37% Chinese Journal of Catalysis 4 publications, 1.37%
Nano Energy	Nano Energy, 4, 1.37% Nano Energy 4 publications, 1.37%
Catalysis Today	Catalysis Today, 4, 1.37% Catalysis Today 4 publications, 1.37%
Advanced Science	Advanced Science, 4, 1.37% Advanced Science 4 publications, 1.37%
ACS Catalysis	ACS Catalysis, 4, 1.37% ACS Catalysis 4 publications, 1.37%
ACS Applied Energy Materials	ACS Applied Energy Materials, 4, 1.37% ACS Applied Energy Materials 4 publications, 1.37%
ACS Applied Nano Materials	ACS Applied Nano Materials, 3, 1.03% ACS Applied Nano Materials 3 publications, 1.03%
Coordination Chemistry Reviews	Coordination Chemistry Reviews, 3, 1.03% Coordination Chemistry Reviews 3 publications, 1.03%
Energy Storage Materials	Energy Storage Materials, 3, 1.03% Energy Storage Materials 3 publications, 1.03%
Journal of Energy Chemistry	Journal of Energy Chemistry, 3, 1.03% Journal of Energy Chemistry 3 publications, 1.03%
Small	Small, 3, 1.03% Small 3 publications, 1.03%
ChemPhysChem	ChemPhysChem, 3, 1.03% ChemPhysChem 3 publications, 1.03%
Chemistry of Materials	Chemistry of Materials, 3, 1.03% Chemistry of Materials 3 publications, 1.03%
Journal of the American Chemical Society	Journal of the American Chemical Society, 3, 1.03% Journal of the American Chemical Society 3 publications, 1.03%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 3, 1.03% Journal of Materials Chemistry C 3 publications, 1.03%
ACS Omega	ACS Omega, 3, 1.03% ACS Omega 3 publications, 1.03%
Physical Review Materials	Physical Review Materials, 2, 0.69% Physical Review Materials 2 publications, 0.69%
	5 10 15 20 25

Citations by publishers

	20 40 60 80 100 120
Elsevier	Elsevier, 103, 35.4% Elsevier 103 publications, 35.4%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 51, 17.53% Royal Society of Chemistry (RSC) 51 publications, 17.53%
Wiley	Wiley, 48, 16.49% Wiley 48 publications, 16.49%
American Chemical Society (ACS)	American Chemical Society (ACS), 48, 16.49% American Chemical Society (ACS) 48 publications, 16.49%
Springer Nature	Springer Nature, 13, 4.47% Springer Nature 13 publications, 4.47%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 5, 1.72% Multidisciplinary Digital Publishing Institute (MDPI) 5 publications, 1.72%
IOP Publishing	IOP Publishing, 5, 1.72% IOP Publishing 5 publications, 1.72%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 3, 1.03% American Institute of Physics (AIP) 3 publications, 1.03%
American Physical Society (APS)	American Physical Society (APS), 3, 1.03% American Physical Society (APS) 3 publications, 1.03%
Walter de Gruyter	Walter de Gruyter, 2, 0.69% Walter de Gruyter 2 publications, 0.69%
The Electrochemical Society	The Electrochemical Society, 1, 0.34% The Electrochemical Society 1 publication, 0.34%
Tsinghua University Press	Tsinghua University Press, 1, 0.34% Tsinghua University Press 1 publication, 0.34%
Taylor & Francis	Taylor & Francis, 1, 0.34% Taylor & Francis 1 publication, 0.34%
Chinese Academy of Sciences	Chinese Academy of Sciences, 1, 0.34% Chinese Academy of Sciences 1 publication, 0.34%
IEEE	IEEE, 1, 0.34% IEEE 1 publication, 0.34%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.34% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.34%
	20 40 60 80 100 120

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Ling C. et al. Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction // Advanced Science. 2016. Vol. 3. No. 11. p. 1600180.

GOST all authors (up to 50) Copy

Ling C., Shi L., Ouyang Y., Chen Q., Wang J. Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction // Advanced Science. 2016. Vol. 3. No. 11. p. 1600180.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1002/advs.201600180

UR - https://doi.org/10.1002/advs.201600180

TI - Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction

T2 - Advanced Science

AU - Shi, Li

AU - Ling, C.

AU - Ouyang, Yixin

AU - Chen, Qian

AU - Wang, Jinlan

PY - 2016

DA - 2016/06/28 00:00:00

PB - Wiley

SP - 1600180

IS - 11

VL - 3

SN - 2198-3844

ER -

BibTex |

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BibTex Copy

@article{2016_Ling,

author = {Li Shi and C. Ling and Yixin Ouyang and Qian Chen and Jinlan Wang},

title = {Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction},

journal = {Advanced Science},

year = {2016},

volume = {3},

publisher = {Wiley},

month = {jun},

url = {https://doi.org/10.1002/advs.201600180},

number = {11},

pages = {1600180},

doi = {10.1002/advs.201600180}

}

MLA

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MLA Copy

Ling, C., et al. “Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction.” Advanced Science, vol. 3, no. 11, Jun. 2016, p. 1600180. https://doi.org/10.1002/advs.201600180.

Found error?

Publisher

Wiley

Journal

Advanced Science

Quartile SCImago

Quartile WOS

Impact factor

15.1

ISSN

21983844 (Print)
21983844 (Electronic)