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Метрики

Издатель

—

Dehydrogenation of Alkanes

Introduction

Importance of Light Alkenes

Historical Developments

Conceptual Approach

Influence of Temperature on the Equilibrium

Influence of Partial Pressure on the Equilibrium

Energy of Alkane Dehydrogenation

Formation of By‐Products

Removal of Hydrogen to Shift the Equilibrium

Spatial Separation of Dehydrogenation and Hydrogen Combustion

Dehydrogenation and Hydrogen Combustion in a Catalyst Bed

Oxidative Dehydrogenation ( ODH )

Catalytic Systems

Supported Chromia Catalysts

Chromia on Al 2 O 3 Supports

A Structure and Reactivity

B Oxidized State

C Reduced State

D Regeneration

Chromia on Si O 2 / Zr O 2 Supports

Supported Platinum/Tin Catalysts

Platinum as Active Component

Tin as Modifier

State and Mode of Operation of Platinum and Tin

A State of Pt and Sn

B Mode of Operation of Pt and Sn

C Ensemble Effect

D Ligand Effect

Role of the Support

Regeneration of Supported Platinum/Tin Catalysts

A Treatment with Molecular Oxygen

B Treatment with Chlorine

C Treatment with Hydrogen

Kinetics and Mechanism

Kinetics of Dehydrogenation

Chromia/Alumina Catalysts

A Mechanism 1

B Mechanism 2

Platinum and Platinum/Tin Catalysts

Kinetics of Deactivation

Reactor Concepts

Endothermic Character

Preheating the Feed and Carrying out the Reaction in an Adiabatic Reaction System

Carrying Out the Reaction in a Heated Reactor

Preheating the Catalyst and Carrying Out the Reaction in an Adiabatic Reactor

Regeneration

Continuous Systems

Discontinuous Systems

Commercial Processes

UOP Oleflex Process

U hde STAR Process

ABB Lummus CATOFIN Process

Linde PDH Process

S namprogetti‐ Y arsintez FBD Process

Dehydrogenation of Other Alkanes

Dehydrogenation of Heavy n ‐Alkanes

Dehydrogenation of Cyclohexane

Future Developments

Membrane Technology

CO 2 as a Diluent

Conclusions and Future Prospects

Новиков Андрей

Винокуров Владимир

Глотов Александр

Топ-30

Журналы

Издатели

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Chromia on Al ₂ O ₃ Supports

Chromia on Si O ₂ / Zr O ₂ Supports

CO ₂ as a Diluent