Open Access
Advanced Science, volume 3, issue 11, pages 1600180
Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction
Publication type: Journal Article
Publication date: 2016-06-28
PubMed ID:
27980992
Medicine (miscellaneous)
General Chemical Engineering
General Physics and Astronomy
General Materials Science
General Engineering
Biochemistry, Genetics and Molecular Biology (miscellaneous)
Abstract
Developing alternatives to precious Pt for hydrogen production from water splitting is central to the area of renewable energy. This work predicts extremely high catalytic activity of transition metal (Fe, Co, and Ni) promoted two-dimensional MXenes, fully oxidized vanadium carbides (V2CO2), for hydrogen evolution reaction (HER). The first-principle calculations show that the introduction of transition metal can greatly weaken the strong binding between hydrogen and oxygen and engineer the hydrogen adsorption free energy to the optimal value ≈0 eV by choosing the suitable type and coverage of the promoters as well as the active sites. Strain engineering on the performance of transition metal promoted V2CO2 further reveals that the excellent HER activities can maintain well while those poor ones can be modulated to be highly active. This study provides new possibilities for cost-effective alternatives to Pt in HER and for the application of 2D MXenes.
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Ling C. et al. Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction // Advanced Science. 2016. Vol. 3. No. 11. p. 1600180.
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Ling C., Shi L., Ouyang Y., Chen Q., Wang J. Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction // Advanced Science. 2016. Vol. 3. No. 11. p. 1600180.
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TY - JOUR
DO - 10.1002/advs.201600180
UR - https://doi.org/10.1002/advs.201600180
TI - Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction
T2 - Advanced Science
AU - Ling, C.
AU - Shi, Li
AU - Ouyang, Yixin
AU - Chen, Qian
AU - Wang, Jinlan
PY - 2016
DA - 2016/06/28
PB - Wiley
SP - 1600180
IS - 11
VL - 3
PMID - 27980992
SN - 2198-3844
ER -
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BibTex (up to 50 authors)
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@article{2016_Ling,
author = {C. Ling and Li Shi and Yixin Ouyang and Qian Chen and Jinlan Wang},
title = {Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction},
journal = {Advanced Science},
year = {2016},
volume = {3},
publisher = {Wiley},
month = {jun},
url = {https://doi.org/10.1002/advs.201600180},
number = {11},
pages = {1600180},
doi = {10.1002/advs.201600180}
}
Cite this
MLA
Copy
Ling, C., et al. “Transition Metal‐Promoted V 2 CO 2 (MXenes): A New and Highly Active Catalyst for Hydrogen Evolution Reaction.” Advanced Science, vol. 3, no. 11, Jun. 2016, p. 1600180. https://doi.org/10.1002/advs.201600180.