Angewandte Chemie - International Edition, volume 57, issue 28, pages 8729-8733
Biomimetic Donor–Acceptor Motifs in Conjugated Polymers for Promoting Exciton Splitting and Charge Separation
Publication type: Journal Article
Publication date: 2018-06-14
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 16.6
ISSN: 14337851, 15213773
General Chemistry
Catalysis
Abstract
Natural photosynthesis serves as a model for energy and chemical conversions, and motivates the search of artificial systems that mimic nature's energy- and electron-transfer chains. However, bioinspired systems often suffer from the partial or even large loss of the charge separation state, and show moderate activity owing to the fundamentally different features of the multiple compounds. Herein, a selenium and cyanamide-functionalized heptazine-based melon (DA-HM) is designed as a unique bioinspired donor-acceptor (D-A) light harvester. The combination of the photosystem and electron shuttle in a single species, with both n- and p-type conductivities, and extended spectral absorption, endows DA-HM with a high efficiency in the transfer and separation of photoexcited charge carriers, resulting in photochemical activity. This work presents a unique conjugated polymeric system that shows great potential for solar-to-chemical conversion by artificial photosynthesis.
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Elsevier
85 publications, 42.29%
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Wiley
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4 publications, 1.99%
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2 publications, 1%
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1 publication, 0.5%
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1 publication, 0.5%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 0.5%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Ou H. et al. Biomimetic Donor–Acceptor Motifs in Conjugated Polymers for Promoting Exciton Splitting and Charge Separation // Angewandte Chemie - International Edition. 2018. Vol. 57. No. 28. pp. 8729-8733.
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Ou H., Chen X., Lin L., Fang Y., Wang X. Biomimetic Donor–Acceptor Motifs in Conjugated Polymers for Promoting Exciton Splitting and Charge Separation // Angewandte Chemie - International Edition. 2018. Vol. 57. No. 28. pp. 8729-8733.
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TY - JOUR
DO - 10.1002/anie.201803863
UR - https://doi.org/10.1002/anie.201803863
TI - Biomimetic Donor–Acceptor Motifs in Conjugated Polymers for Promoting Exciton Splitting and Charge Separation
T2 - Angewandte Chemie - International Edition
AU - Ou, Honghui
AU - Chen, Xinru
AU - Wang, Xinchen
AU - Lin, Li-Hua
AU - Fang, Yuanxing
PY - 2018
DA - 2018/06/14 00:00:00
PB - Wiley
SP - 8729-8733
IS - 28
VL - 57
SN - 1433-7851
SN - 1521-3773
ER -
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@article{2018_Ou,
author = {Honghui Ou and Xinru Chen and Xinchen Wang and Li-Hua Lin and Yuanxing Fang},
title = {Biomimetic Donor–Acceptor Motifs in Conjugated Polymers for Promoting Exciton Splitting and Charge Separation},
journal = {Angewandte Chemie - International Edition},
year = {2018},
volume = {57},
publisher = {Wiley},
month = {jun},
url = {https://doi.org/10.1002/anie.201803863},
number = {28},
pages = {8729--8733},
doi = {10.1002/anie.201803863}
}
Cite this
MLA
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Ou, Honghui, et al. “Biomimetic Donor–Acceptor Motifs in Conjugated Polymers for Promoting Exciton Splitting and Charge Separation.” Angewandte Chemie - International Edition, vol. 57, no. 28, Jun. 2018, pp. 8729-8733. https://doi.org/10.1002/anie.201803863.