Advanced Functional Materials, volume 27, issue 2, pages 1603605

Synergistic Effect of Hybrid PbS Quantum Dots/2D-WSe₂Toward High Performance and Broadband Phototransistors

Chao Hu ¹

Dongdong Dong ¹

Xiaokun Yang ¹

Keke Qiao ¹

Dun Yang ¹

Hui Deng ¹

Shengjie Yuan ¹

Jahangeer Khan ¹

Lan Yang ¹

Haisheng Song ¹

Jiang Hong Tang ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

Wuhan National Laboratory for Optoelectronics (WNLO) and School of Optical and Electronic Information; Huazhong University of Science and Technology; 1037 Luoyu Road Wuhan Hubei 430074 P. R. China |

Publication type: Journal Article

Publication date: 2016-11-16

Wiley

Journal: Advanced Functional Materials

Quartile SCImago

Quartile WOS

Impact factor: 19

ISSN: 1616301X, 16163028

DOI: 10.1002/adfm.201603605

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Electronic, Optical and Magnetic Materials

Electrochemistry

Condensed Matter Physics

Biomaterials

Abstract

The transitionmetal dichalcogenides-based phototransistors have demonstrated high transport mobility but are limited to poor photoresponse, which greatly blocks their applications in optoelectronic fields. Here, light sensitive PbS colloidal quantum dots (QDs) combined with 2D WSe2 to develop hybrid QDs/2D-WSe2 phototransistors for high performance and broadband photodetection are utilized. The device shows a responsivity up to 2 × 105 A W–1, which is orders of magnitude higher than the counterpart of individual material-based devices. The detection spectra of hybrid devices can be extended to near infrared similar to QDs' response. The high performance of hybrid 0D-2D phototransistor is ascribed to the synergistic function of photogating effect. PbS QDs can efficiently absorb the input illumination and 2D WSe2 supports a transport expressway for injected photocarriers. The hybrid phototransistors obtain a specific detectivity over 1013 Jones in both ON and OFF state in contrast to the depleted working state (OFF) for other reported QDs/2D phototransistors. The present device construction strategy, photogating enhanced performance, and robust device working conditions contain high potential for future optoelectronic devices.

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Materials and Design	Materials and Design, 2, 1% Materials and Design 2 publications, 1%
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	2 4 6 8 10 12 14 16 18

Citations by publishers

	5 10 15 20 25 30 35 40 45
Wiley	Wiley, 45, 22.39% Wiley 45 publications, 22.39%
American Chemical Society (ACS)	American Chemical Society (ACS), 44, 21.89% American Chemical Society (ACS) 44 publications, 21.89%
Elsevier	Elsevier, 28, 13.93% Elsevier 28 publications, 13.93%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 21, 10.45% Royal Society of Chemistry (RSC) 21 publications, 10.45%
Springer Nature	Springer Nature, 14, 6.97% Springer Nature 14 publications, 6.97%
IOP Publishing	IOP Publishing, 13, 6.47% IOP Publishing 13 publications, 6.47%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 10, 4.98% American Institute of Physics (AIP) 10 publications, 4.98%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 7, 3.48% Multidisciplinary Digital Publishing Institute (MDPI) 7 publications, 3.48%
American Physical Society (APS)	American Physical Society (APS), 4, 1.99% American Physical Society (APS) 4 publications, 1.99%
Frontiers Media S.A.	Frontiers Media S.A., 2, 1% Frontiers Media S.A. 2 publications, 1%
Pleiades Publishing	Pleiades Publishing, 2, 1% Pleiades Publishing 2 publications, 1%
Optical Society of America	Optical Society of America, 2, 1% Optical Society of America 2 publications, 1%
Bentham Science	Bentham Science, 1, 0.5% Bentham Science 1 publication, 0.5%
Cambridge University Press	Cambridge University Press, 1, 0.5% Cambridge University Press 1 publication, 0.5%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.5% American Association for the Advancement of Science (AAAS) 1 publication, 0.5%
Opto-Electronic Advances	Opto-Electronic Advances, 1, 0.5% Opto-Electronic Advances 1 publication, 0.5%
Chinese Physical Society	Chinese Physical Society, 1, 0.5% Chinese Physical Society 1 publication, 0.5%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.5% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.5%
	5 10 15 20 25 30 35 40 45

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Hu C. et al. Synergistic Effect of Hybrid PbS Quantum Dots/2D-WSe2Toward High Performance and Broadband Phototransistors // Advanced Functional Materials. 2016. Vol. 27. No. 2. p. 1603605.

GOST all authors (up to 50) Copy

Hu C., Dong D., Yang X., Qiao K., Yang D., Deng H., Yuan S., Khan J., Yang L., Song H., Tang J. H. Synergistic Effect of Hybrid PbS Quantum Dots/2D-WSe2Toward High Performance and Broadband Phototransistors // Advanced Functional Materials. 2016. Vol. 27. No. 2. p. 1603605.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1002/adfm.201603605

UR - https://doi.org/10.1002/adfm.201603605

TI - Synergistic Effect of Hybrid PbS Quantum Dots/2D-WSe2Toward High Performance and Broadband Phototransistors

T2 - Advanced Functional Materials

AU - Dong, Dongdong

AU - Yang, Xiaokun

AU - Qiao, Keke

AU - Yang, Dun

AU - Deng, Hui

AU - Yuan, Shengjie

AU - Khan, Jahangeer

AU - Yang, Lan

AU - Hu, Chao

AU - Song, Haisheng

AU - Tang, Jiang Hong

PY - 2016

DA - 2016/11/16 00:00:00

PB - Wiley

SP - 1603605

IS - 2

VL - 27

SN - 1616-301X

SN - 1616-3028

ER -

BibTex |

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BibTex Copy

@article{2016_Hu,

author = {Dongdong Dong and Xiaokun Yang and Keke Qiao and Dun Yang and Hui Deng and Shengjie Yuan and Jahangeer Khan and Lan Yang and Chao Hu and Haisheng Song and Jiang Hong Tang},

title = {Synergistic Effect of Hybrid PbS Quantum Dots/2D-WSe2Toward High Performance and Broadband Phototransistors},

journal = {Advanced Functional Materials},

year = {2016},

volume = {27},

publisher = {Wiley},

month = {nov},

url = {https://doi.org/10.1002/adfm.201603605},

number = {2},

pages = {1603605},

doi = {10.1002/adfm.201603605}

}

MLA

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Hu, Chao, et al. “Synergistic Effect of Hybrid PbS Quantum Dots/2D-WSe2Toward High Performance and Broadband Phototransistors.” Advanced Functional Materials, vol. 27, no. 2, Nov. 2016, p. 1603605. https://doi.org/10.1002/adfm.201603605.

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Publisher

Wiley

Journal

Advanced Functional Materials

Quartile SCImago

Quartile WOS

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1616301X (Print)
16163028 (Electronic)