Tuning of the Optical, Electronic, and Magnetic Properties of Boron Nitride Nanosheets with Oxygen Doping and Functionalization
Qunhong Weng
1
,
Dmitry Kvashnin
2
,
Xi Wang
3
,
Ovidiu Cretu
1
,
Yijun Yang
3
,
Min Zhou
1
,
Chao Zhang
1, 4
,
Daiming Tang
1
,
Pavel B. Sorokin
2, 5
,
Yoshio Bando
1
,
Dmitri Golberg
1, 4
Publication type: Journal Article
Publication date: 2017-05-19
scimago Q1
wos Q1
SJR: 8.851
CiteScore: 39.4
Impact factor: 26.8
ISSN: 09359648, 15214095
PubMed ID:
28523720
General Materials Science
Mechanical Engineering
Mechanics of Materials
Abstract
Engineering of the optical, electronic, and magnetic properties of hexagonal boron nitride (h-BN) nanomaterials via oxygen doping and functionalization has been envisaged in theory. However, it is still unclear as to what extent these properties can be altered using such methodology because of the lack of significant experimental progress and systematic theoretical investigations. Therefore, here, comprehensive theoretical predictions verified by solid experimental confirmations are provided, which unambiguously answer this long-standing question. Narrowing of the optical bandgap in h-BN nanosheets (from ≈5.5 eV down to 2.1 eV) and the appearance of paramagnetism and photoluminescence (of both Stokes and anti-Stokes types) in them after oxygen doping and functionalization are discussed. These results are highly valuable for further advances in semiconducting nanoscale electronics, optoelectronics, and spintronics.
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Total citations:
206
Citations from 2024:
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Weng Q. et al. Tuning of the Optical, Electronic, and Magnetic Properties of Boron Nitride Nanosheets with Oxygen Doping and Functionalization // Advanced Materials. 2017. Vol. 29. No. 28. p. 1700695.
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Weng Q., Kvashnin D., Wang X., Cretu O., Yang Y., Zhou M., Zhang C., Tang D., Sorokin P. B., Bando Y., Golberg D. Tuning of the Optical, Electronic, and Magnetic Properties of Boron Nitride Nanosheets with Oxygen Doping and Functionalization // Advanced Materials. 2017. Vol. 29. No. 28. p. 1700695.
Cite this
RIS
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TY - JOUR
DO - 10.1002/adma.201700695
UR - https://doi.org/10.1002/adma.201700695
TI - Tuning of the Optical, Electronic, and Magnetic Properties of Boron Nitride Nanosheets with Oxygen Doping and Functionalization
T2 - Advanced Materials
AU - Weng, Qunhong
AU - Kvashnin, Dmitry
AU - Wang, Xi
AU - Cretu, Ovidiu
AU - Yang, Yijun
AU - Zhou, Min
AU - Zhang, Chao
AU - Tang, Daiming
AU - Sorokin, Pavel B.
AU - Bando, Yoshio
AU - Golberg, Dmitri
PY - 2017
DA - 2017/05/19
PB - Wiley
SP - 1700695
IS - 28
VL - 29
PMID - 28523720
SN - 0935-9648
SN - 1521-4095
ER -
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BibTex (up to 50 authors)
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@article{2017_Weng,
author = {Qunhong Weng and Dmitry Kvashnin and Xi Wang and Ovidiu Cretu and Yijun Yang and Min Zhou and Chao Zhang and Daiming Tang and Pavel B. Sorokin and Yoshio Bando and Dmitri Golberg},
title = {Tuning of the Optical, Electronic, and Magnetic Properties of Boron Nitride Nanosheets with Oxygen Doping and Functionalization},
journal = {Advanced Materials},
year = {2017},
volume = {29},
publisher = {Wiley},
month = {may},
url = {https://doi.org/10.1002/adma.201700695},
number = {28},
pages = {1700695},
doi = {10.1002/adma.201700695}
}
Cite this
MLA
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Weng, Qunhong, et al. “Tuning of the Optical, Electronic, and Magnetic Properties of Boron Nitride Nanosheets with Oxygen Doping and Functionalization.” Advanced Materials, vol. 29, no. 28, May. 2017, p. 1700695. https://doi.org/10.1002/adma.201700695.