Advanced Materials, volume 34, issue 32, pages 2202143
Ion–Dipole Interaction Regulation Enables High‐Performance Single‐Ion Polymer Conductors for Solid‐State Batteries
Publication type: Journal Article
Publication date: 2022-07-10
Journal:
Advanced Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 29.4
ISSN: 09359648, 15214095
General Materials Science
Mechanical Engineering
Mechanics of Materials
Abstract
Solid polymer electrolytes with large ionic conductivity, high ionic transference number, and good interfacial compatibility with electrodes are highly desired for solid-state batteries. However, unwanted polarizations and side reactions occurring in traditional dual-ion polymer conductors hinder their practical applications. Here, single-ion polymer conductors (SIPCs) with exceptional selectivity for Li-ion conduction (Li-ion transference number up to 0.93), high room-temperature ionic conductivity of about 10-4 S cm-1 , and a wide electrochemical stability window (>4.5 V, vs Li/Li+ ) are prepared by precisely regulating the ion-dipole interactions between Li+ and carbonyl/cyano groups. The resulting SIPCs show an excellent electrochemical stability with Li metal during long-term cycling at room temperature and 60 °C. LiFePO4 -based solid-state cells containing the SIPCs exhibit good rate and cycling performance in a wide temperature range from -20 to 90 °C. By the same way of ion-dipole interaction regulation, sodium- and potassium-based SIPCs with both high ionic conductivity and high cationic transference numbers are also prepared. The findings in this work provide guidance for the development of high-performance SIPCs and other metal-ion systems beyond Li+ .
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Citations by publishers
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Wiley
42 publications, 56%
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15 publications, 20%
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3 publications, 4%
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1 publication, 1.33%
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5
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35
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Wen K. et al. Ion–Dipole Interaction Regulation Enables High‐Performance Single‐Ion Polymer Conductors for Solid‐State Batteries // Advanced Materials. 2022. Vol. 34. No. 32. p. 2202143.
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Wen K., Xin C., Guan S., Wu X., Shan H., Xue C., Liu S., Shen Y., Li L., Nan C. Ion–Dipole Interaction Regulation Enables High‐Performance Single‐Ion Polymer Conductors for Solid‐State Batteries // Advanced Materials. 2022. Vol. 34. No. 32. p. 2202143.
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TY - JOUR
DO - 10.1002/adma.202202143
UR - https://doi.org/10.1002/adma.202202143
TI - Ion–Dipole Interaction Regulation Enables High‐Performance Single‐Ion Polymer Conductors for Solid‐State Batteries
T2 - Advanced Materials
AU - Wen, Kaihua
AU - Xin, Chengzhou
AU - Guan, Shundong
AU - Wu, Xinbin
AU - Shan, He
AU - Xue, Chuanjiao
AU - Liu, Sijie
AU - Nan, Ce-Wen
AU - Li, Liangliang
AU - Shen, Yang
PY - 2022
DA - 2022/07/10 00:00:00
PB - Wiley
SP - 2202143
IS - 32
VL - 34
SN - 0935-9648
SN - 1521-4095
ER -
Cite this
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@article{2022_Wen,
author = {Kaihua Wen and Chengzhou Xin and Shundong Guan and Xinbin Wu and He Shan and Chuanjiao Xue and Sijie Liu and Ce-Wen Nan and Liangliang Li and Yang Shen},
title = {Ion–Dipole Interaction Regulation Enables High‐Performance Single‐Ion Polymer Conductors for Solid‐State Batteries},
journal = {Advanced Materials},
year = {2022},
volume = {34},
publisher = {Wiley},
month = {jul},
url = {https://doi.org/10.1002/adma.202202143},
number = {32},
pages = {2202143},
doi = {10.1002/adma.202202143}
}
Cite this
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Wen, Kaihua, et al. “Ion–Dipole Interaction Regulation Enables High‐Performance Single‐Ion Polymer Conductors for Solid‐State Batteries.” Advanced Materials, vol. 34, no. 32, Jul. 2022, p. 2202143. https://doi.org/10.1002/adma.202202143.