Advanced Synthesis and Catalysis

, том 356 , издание 4 , страницы 771-780

Unprecedented control of selectivity in Nickel-catalyzed hydrophosphorylation of alkynes: Efficient route to mono- and bisphosphonates

Тип публикации: Journal Article

Дата публикации: 2014-03-03

Wiley

Advanced Synthesis and Catalysis

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WOS Q1

БС1

SJR: 0.704

CiteScore: 6.9

Impact factor: 3.7

ISSN: 16154150, 16154169

DOI: 10.1002/adsc.201400123

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General Chemistry

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Received: February 3, 2014; Published online: March 3, 2014Dedicated to the memory of Z. A. Starikova.Supporting information for this article is available on the WWW under http://dx.doi.org/10.1002/adsc.201400123.Abstract: A unique nickel-based catalytic system wasdeveloped where the direction of the hydrophos-phorylation reaction can be controlled by varyingthe catalyst loading. A flexible one-pot access to vi-nylmonophosphonates and alkylbisphosphonates wasdemonstrated using simple starting materials in anatom-economic reaction without any specific solventsor ligands. Monitoring of the reaction mechanismwith joint NMR and MS studies revealed key infor-mation about the reaction intermediates. The syn-thetic scope of the developed catalytic system wasexplored and the utility of the synthesized productsfor the fire protection of cotton materials was dem-onstrated.Keywords: alkynes; homogeneous catalysis; nickel;phosphorylation; selectivity

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Khemchyan L. L. et al. Unprecedented control of selectivity in Nickel-catalyzed hydrophosphorylation of alkynes: Efficient route to mono- and bisphosphonates // Advanced Synthesis and Catalysis. 2014. Vol. 356. No. 4. pp. 771-780.

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Khemchyan L. L., Ivanova J. V., S. Zalesskiy S., Ananikov V. P., Beletskaya I. P., Starikova Z. A. Unprecedented control of selectivity in Nickel-catalyzed hydrophosphorylation of alkynes: Efficient route to mono- and bisphosphonates // Advanced Synthesis and Catalysis. 2014. Vol. 356. No. 4. pp. 771-780.

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TY - JOUR

DO - 10.1002/adsc.201400123

UR - https://doi.org/10.1002/adsc.201400123

TI - Unprecedented control of selectivity in Nickel-catalyzed hydrophosphorylation of alkynes: Efficient route to mono- and bisphosphonates

T2 - Advanced Synthesis and Catalysis

AU - Khemchyan, Levon L

AU - Ivanova, Julia V

AU - S. Zalesskiy, Sergey

AU - Ananikov, Valentine P

AU - Beletskaya, Irina P.

AU - Starikova, Zoya A.

PY - 2014

DA - 2014/03/03

PB - Wiley

SP - 771-780

IS - 4

VL - 356

SN - 1615-4150

SN - 1615-4169

ER -

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@article{2014_Khemchyan,

author = {Levon L Khemchyan and Julia V Ivanova and Sergey S. Zalesskiy and Valentine P Ananikov and Irina P. Beletskaya and Zoya A. Starikova},

title = {Unprecedented control of selectivity in Nickel-catalyzed hydrophosphorylation of alkynes: Efficient route to mono- and bisphosphonates},

journal = {Advanced Synthesis and Catalysis},

year = {2014},

volume = {356},

publisher = {Wiley},

month = {mar},

url = {https://doi.org/10.1002/adsc.201400123},

number = {4},

pages = {771--780},

doi = {10.1002/adsc.201400123}

}

MLA

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MLA Скопировать

Khemchyan, Levon L., et al. “Unprecedented control of selectivity in Nickel-catalyzed hydrophosphorylation of alkynes: Efficient route to mono- and bisphosphonates.” Advanced Synthesis and Catalysis, vol. 356, no. 4, Mar. 2014, pp. 771-780. https://doi.org/10.1002/adsc.201400123.

Издатель

Wiley

Журнал

Advanced Synthesis and Catalysis

SCImago Q1

WOS Q1

БС1

SJR

0.704

CiteScore

6.9

Impact factor