Open Access
Advanced Science, volume 4, issue 8, pages 1600517
Strategies Based on Nitride Materials Chemistry to Stabilize Li Metal Anode
Publication type: Journal Article
Publication date: 2017-03-03
Journal:
Advanced Science
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 15.1
ISSN: 21983844, 21983844
Medicine (miscellaneous)
General Chemical Engineering
General Physics and Astronomy
General Materials Science
General Engineering
Biochemistry, Genetics and Molecular Biology (miscellaneous)
Abstract
Lithium metal battery is a promising candidate for high-energy-density energy storage. Unfortunately, the strongly reducing nature of lithium metal has been an outstanding challenge causing poor stability and low coulombic efficiency in lithium batteries. For decades, there are significant research efforts to stabilize lithium metal anode. However, such efforts are greatly impeded by the lack of knowledge about lithium-stable materials chemistry. So far, only a few materials are known to be stable against Li metal. To resolve this outstanding challenge, lithium-stable materials have been uncovered out of chemistry across the periodic table using first-principles calculations based on large materials database. It is found that most oxides, sulfides, and halides, commonly studied as protection materials, are reduced by lithium metal due to the reduction of metal cations. It is discovered that nitride anion chemistry exhibits unique stability against Li metal, which is either thermodynamically intrinsic or a result of stable passivation. The results here establish essential guidelines for selecting, designing, and discovering materials for lithium metal protection, and propose multiple novel strategies of using nitride materials and high nitrogen doping to form stable solid-electrolyte-interphase for lithium metal anode, paving the way for high-energy rechargeable lithium batteries.
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Citations by publishers
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Wiley
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2 publications, 1%
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2 publications, 1%
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1 publication, 0.5%
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1 publication, 0.5%
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1 publication, 0.5%
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1 publication, 0.5%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Zhu Y. et al. Strategies Based on Nitride Materials Chemistry to Stabilize Li Metal Anode // Advanced Science. 2017. Vol. 4. No. 8. p. 1600517.
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Zhu Y., He X., Mo Y. Strategies Based on Nitride Materials Chemistry to Stabilize Li Metal Anode // Advanced Science. 2017. Vol. 4. No. 8. p. 1600517.
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TY - JOUR
DO - 10.1002/advs.201600517
UR - https://doi.org/10.1002/advs.201600517
TI - Strategies Based on Nitride Materials Chemistry to Stabilize Li Metal Anode
T2 - Advanced Science
AU - Zhu, Yizhou
AU - He, Xingfeng
AU - Mo, Yifei
PY - 2017
DA - 2017/03/03 00:00:00
PB - Wiley
SP - 1600517
IS - 8
VL - 4
SN - 2198-3844
SN - 2198-3844
ER -
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@article{2017_Zhu,
author = {Yizhou Zhu and Xingfeng He and Yifei Mo},
title = {Strategies Based on Nitride Materials Chemistry to Stabilize Li Metal Anode},
journal = {Advanced Science},
year = {2017},
volume = {4},
publisher = {Wiley},
month = {mar},
url = {https://doi.org/10.1002/advs.201600517},
number = {8},
pages = {1600517},
doi = {10.1002/advs.201600517}
}
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MLA
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Zhu, Yizhou, et al. “Strategies Based on Nitride Materials Chemistry to Stabilize Li Metal Anode.” Advanced Science, vol. 4, no. 8, Mar. 2017, p. 1600517. https://doi.org/10.1002/advs.201600517.