Advanced Energy Materials, volume 11, issue 14, pages 2003836
Single‐Ion Conducting Polymer Electrolytes for Solid‐State Lithium–Metal Batteries: Design, Performance, and Challenges
2
Department of Chemistry University of Tennessee Knoxville TN 37996 USA
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4
Bredesen Center for Interdisciplinary Research and Graduate Education University of Tennessee Knoxville TN 37996 USA
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Publication type: Journal Article
Publication date: 2021-02-28
Journal:
Advanced Energy Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 27.8
ISSN: 16146832, 16146840
General Materials Science
Renewable Energy, Sustainability and the Environment
Abstract
Realizing solid-state lithium batteries with higher energy density and enhanced safety compared to the conventional liquid lithium-ion batteries is one of the primary research and development goals set for next-generation batteries in this decade. In this regard, polymer electrolytes have been widely researched as solid electrolytes due to their excellent processability, flexibility, and low weight. With high cationic transference numbers (tLi+ close to 1), single-ion conducting polymer electrolytes (SICPEs) have tremendous advantages compared to polymer electrolyte systems (tLi+ < 0.4) because of their potential to reduce the buildup of ion concentration gradients and suppress growth of lithium dendrites. The current review covers the fundamentals of SICPEs, including anionic unit synthesis, polymer structure design, and film fabrication, along with simulation and experimental results in solid-state lithium–metal battery applications. A perspective on current challenges, possible solutions, and potential research directions of SICPEs is also discussed to provide the research community with the critical technical aspects that may advance SICPEs as solid electrolytes in next-generation energy storage systems.
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Citations by publishers
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Wiley
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1 publication, 0.44%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 0.44%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Zhu J. et al. Single‐Ion Conducting Polymer Electrolytes for Solid‐State Lithium–Metal Batteries: Design, Performance, and Challenges // Advanced Energy Materials. 2021. Vol. 11. No. 14. p. 2003836.
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Zhu J., Zhang Z., Zhao S., Tepavcevic S., Belharouak I., Cao P. Single‐Ion Conducting Polymer Electrolytes for Solid‐State Lithium–Metal Batteries: Design, Performance, and Challenges // Advanced Energy Materials. 2021. Vol. 11. No. 14. p. 2003836.
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TY - JOUR
DO - 10.1002/aenm.202003836
UR - https://doi.org/10.1002/aenm.202003836
TI - Single‐Ion Conducting Polymer Electrolytes for Solid‐State Lithium–Metal Batteries: Design, Performance, and Challenges
T2 - Advanced Energy Materials
AU - Zhao, Sheng
AU - Cao, Pengfei
AU - Zhu, Jiadeng
AU - Zhang, Zhen
AU - Tepavcevic, Sanja
AU - Belharouak, Ilias
PY - 2021
DA - 2021/02/28 00:00:00
PB - Wiley
SP - 2003836
IS - 14
VL - 11
SN - 1614-6832
SN - 1614-6840
ER -
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@article{2021_Zhu,
author = {Sheng Zhao and Pengfei Cao and Jiadeng Zhu and Zhen Zhang and Sanja Tepavcevic and Ilias Belharouak},
title = {Single‐Ion Conducting Polymer Electrolytes for Solid‐State Lithium–Metal Batteries: Design, Performance, and Challenges},
journal = {Advanced Energy Materials},
year = {2021},
volume = {11},
publisher = {Wiley},
month = {feb},
url = {https://doi.org/10.1002/aenm.202003836},
number = {14},
pages = {2003836},
doi = {10.1002/aenm.202003836}
}
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MLA
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Zhu, Jiadeng, et al. “Single‐Ion Conducting Polymer Electrolytes for Solid‐State Lithium–Metal Batteries: Design, Performance, and Challenges.” Advanced Energy Materials, vol. 11, no. 14, Feb. 2021, p. 2003836. https://doi.org/10.1002/aenm.202003836.