Advanced Energy Materials, volume 11, issue 24, pages 2100654

Influence of Crystallinity of Lithium Thiophosphate Solid Electrolytes on the Performance of Solid‐State Batteries

Shuo Wang ^{1, 2}

Wenbo Zhang ¹

Xiang Chen ³

Dyuman Das ¹

Raffael Rueß ¹

Ajay Gautam ¹

Felix Walther ¹

Saneyuki Ohno ¹

Raimund Koerver ¹

Qiang Zhang ³

WOLFGANG G. ZEIER ⁴

Felix H. Richter ¹

Ce-Wen Nan ²

Jürgen Janek ¹

Hide authors affiliations Show authors affiliations: 4 affiliations

Institute of Physical Chemistry & Center for Materials Research Justus‐Liebig‐University Giessen Heinrich‐Buff‐Ring 17 Giessen D‐35392 Germany |

State Key Laboratory of New Ceramics and Fine processing School of Materials Science and Engineering Tsinghua University Beijing 100084 China |

Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical Engineering Tsinghua University Beijing 100084 China |

⁴

Institute of Inorganic and Analytical Chemistry University of Münster Corrensstrasse 30 Muenster 48149 Germany |

Publication type: Journal Article

Publication date: 2021-05-06

Wiley

Journal: Advanced Energy Materials

Quartile SCImago

Quartile WOS

Impact factor: 27.8

ISSN: 16146832, 16146840

DOI: 10.1002/aenm.202100654

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Abstract

Solid electrolytes (SEs) largely define the properties of all‐solid‐state batteries (ASSBs) and are expected to improve their safety, stability, and performance. Their ionic conductivity has much improved in recent years, enabling higher power and energy density. However, more subtle parameters, such as crystallinity, may also influence the electrochemical performance of cells. In this work, the correlation between the performance of ASSBs and thiophosphate SEs having the same stoichiometry, but different crystallinity is investigated. In In/InLi | SE | LiCoO2@ LiNb0.5Ta0.5O3 model cells, better cycling and rate performance is achieved when using glass/glass‐ceramic SEs (e.g., 75Li2S·25P2S5 glass, 70Li2S·30P2S5 glass, and Li6PS5Cl glass‐ceramic). This can be mostly attributed to the mitigation of contact loss by the glass/glass‐ceramic SEs compared to their crystalline SE counterparts. Furthermore, the SE decomposition at typical cathode potentials is investigated by using SE and carbon composites as cathodes. Larger volume changes and more severe decomposition are observed with crystalline SEs in the SE/carbon composite cathode after cycling. The crystalline SEs show higher electronic partial conductivity which results in more degradation in the composite cathode. This work sheds light on optimized composite cathode design for ASSB by carefully choosing solid electrolytes with appropriate mechanical and (electro‐)chemical properties.

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Citations by journals

	1 2 3 4 5 6 7 8
Advanced Energy Materials	Advanced Energy Materials, 8, 10.39% Advanced Energy Materials 8 publications, 10.39%
Advanced Functional Materials	Advanced Functional Materials, 5, 6.49% Advanced Functional Materials 5 publications, 6.49%
ACS applied materials & interfaces	ACS applied materials & interfaces, 3, 3.9% ACS applied materials & interfaces 3 publications, 3.9%
Chemistry of Materials	Chemistry of Materials, 3, 3.9% Chemistry of Materials 3 publications, 3.9%
Batteries	Batteries, 3, 3.9% Batteries 3 publications, 3.9%
ACS Applied Energy Materials	ACS Applied Energy Materials, 3, 3.9% ACS Applied Energy Materials 3 publications, 3.9%
ACS Energy Letters	ACS Energy Letters, 3, 3.9% ACS Energy Letters 3 publications, 3.9%
Advanced Materials Interfaces	Advanced Materials Interfaces, 2, 2.6% Advanced Materials Interfaces 2 publications, 2.6%
Advanced Energy and Sustainability Research	Advanced Energy and Sustainability Research, 2, 2.6% Advanced Energy and Sustainability Research 2 publications, 2.6%
Chemical Engineering Journal	Chemical Engineering Journal, 2, 2.6% Chemical Engineering Journal 2 publications, 2.6%
Materials Futures	Materials Futures, 2, 2.6% Materials Futures 2 publications, 2.6%
Batteries & Supercaps	Batteries & Supercaps, 2, 2.6% Batteries & Supercaps 2 publications, 2.6%
ChemSusChem	ChemSusChem, 2, 2.6% ChemSusChem 2 publications, 2.6%
Energy and Environmental Science	Energy and Environmental Science, 2, 2.6% Energy and Environmental Science 2 publications, 2.6%
Journal of the American Chemical Society	Journal of the American Chemical Society, 2, 2.6% Journal of the American Chemical Society 2 publications, 2.6%
ACS Sustainable Chemistry and Engineering	ACS Sustainable Chemistry and Engineering, 1, 1.3% ACS Sustainable Chemistry and Engineering 1 publication, 1.3%
Applied Physics Letters	Applied Physics Letters, 1, 1.3% Applied Physics Letters 1 publication, 1.3%
Journal of Electronic Materials	Journal of Electronic Materials, 1, 1.3% Journal of Electronic Materials 1 publication, 1.3%
Frontiers in Chemical Engineering	Frontiers in Chemical Engineering, 1, 1.3% Frontiers in Chemical Engineering 1 publication, 1.3%
Scientific Reports	Scientific Reports, 1, 1.3% Scientific Reports 1 publication, 1.3%
Journal of Solid State Electrochemistry	Journal of Solid State Electrochemistry, 1, 1.3% Journal of Solid State Electrochemistry 1 publication, 1.3%
Rare Metals	Rare Metals, 1, 1.3% Rare Metals 1 publication, 1.3%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 1, 1.3% Journal of Materials Chemistry A 1 publication, 1.3%
Current Opinion in Solid State and Materials Science	Current Opinion in Solid State and Materials Science, 1, 1.3% Current Opinion in Solid State and Materials Science 1 publication, 1.3%
Particuology	Particuology, 1, 1.3% Particuology 1 publication, 1.3%
Small Structures	Small Structures, 1, 1.3% Small Structures 1 publication, 1.3%
InfoMat	InfoMat, 1, 1.3% InfoMat 1 publication, 1.3%
Energy Technology	Energy Technology, 1, 1.3% Energy Technology 1 publication, 1.3%
Electrochemistry	Electrochemistry, 1, 1.3% Electrochemistry 1 publication, 1.3%
Materials Advances	Materials Advances, 1, 1.3% Materials Advances 1 publication, 1.3%
	1 2 3 4 5 6 7 8

Citations by publishers

	5 10 15 20 25 30
Wiley	Wiley, 28, 36.36% Wiley 28 publications, 36.36%
American Chemical Society (ACS)	American Chemical Society (ACS), 16, 20.78% American Chemical Society (ACS) 16 publications, 20.78%
Elsevier	Elsevier, 8, 10.39% Elsevier 8 publications, 10.39%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 6, 7.79% Royal Society of Chemistry (RSC) 6 publications, 7.79%
Springer Nature	Springer Nature, 4, 5.19% Springer Nature 4 publications, 5.19%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 4, 5.19% Multidisciplinary Digital Publishing Institute (MDPI) 4 publications, 5.19%
IOP Publishing	IOP Publishing, 2, 2.6% IOP Publishing 2 publications, 2.6%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 1.3% American Institute of Physics (AIP) 1 publication, 1.3%
Frontiers Media S.A.	Frontiers Media S.A., 1, 1.3% Frontiers Media S.A. 1 publication, 1.3%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 1.3% Nonferrous Metals Society of China 1 publication, 1.3%
The Electrochemical Society of Japan	The Electrochemical Society of Japan, 1, 1.3% The Electrochemical Society of Japan 1 publication, 1.3%
American Vacuum Society	American Vacuum Society, 1, 1.3% American Vacuum Society 1 publication, 1.3%
The Electrochemical Society	The Electrochemical Society, 1, 1.3% The Electrochemical Society 1 publication, 1.3%
OAE Publishing Inc.	OAE Publishing Inc., 1, 1.3% OAE Publishing Inc. 1 publication, 1.3%
Chinese Academy of Sciences	Chinese Academy of Sciences, 1, 1.3% Chinese Academy of Sciences 1 publication, 1.3%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.3% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.3%
	5 10 15 20 25 30

We do not take into account publications without a DOI.
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GOST Copy

Wang S. et al. Influence of Crystallinity of Lithium Thiophosphate Solid Electrolytes on the Performance of Solid‐State Batteries // Advanced Energy Materials. 2021. Vol. 11. No. 24. p. 2100654.

GOST all authors (up to 50) Copy

Wang S., Zhang W., Chen X., Das D., Rueß R., Gautam A., Walther F., Ohno S., Koerver R., Zhang Q., ZEIER W. G., Richter F. H., Nan C., Janek J. Influence of Crystallinity of Lithium Thiophosphate Solid Electrolytes on the Performance of Solid‐State Batteries // Advanced Energy Materials. 2021. Vol. 11. No. 24. p. 2100654.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1002/aenm.202100654

UR - https://doi.org/10.1002/aenm.202100654

TI - Influence of Crystallinity of Lithium Thiophosphate Solid Electrolytes on the Performance of Solid‐State Batteries

T2 - Advanced Energy Materials

AU - Wang, Shuo

AU - Zhang, Wenbo

AU - Chen, Xiang

AU - Das, Dyuman

AU - Rueß, Raffael

AU - Gautam, Ajay

AU - Walther, Felix

AU - Ohno, Saneyuki

AU - Koerver, Raimund

AU - Zhang, Qiang

AU - ZEIER, WOLFGANG G.

AU - Richter, Felix H.

AU - Nan, Ce-Wen

AU - Janek, Jürgen

PY - 2021

DA - 2021/05/06 00:00:00

PB - Wiley

SP - 2100654

IS - 24

VL - 11

SN - 1614-6832

SN - 1614-6840

ER -

BibTex |

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BibTex Copy

@article{2021_Wang,

author = {Shuo Wang and Wenbo Zhang and Xiang Chen and Dyuman Das and Raffael Rueß and Ajay Gautam and Felix Walther and Saneyuki Ohno and Raimund Koerver and Qiang Zhang and WOLFGANG G. ZEIER and Felix H. Richter and Ce-Wen Nan and Jürgen Janek},

title = {Influence of Crystallinity of Lithium Thiophosphate Solid Electrolytes on the Performance of Solid‐State Batteries},

journal = {Advanced Energy Materials},

year = {2021},

volume = {11},

publisher = {Wiley},

month = {may},

url = {https://doi.org/10.1002/aenm.202100654},

number = {24},

pages = {2100654},

doi = {10.1002/aenm.202100654}

}

MLA

Cite this

MLA Copy

Wang, Shuo, et al. “Influence of Crystallinity of Lithium Thiophosphate Solid Electrolytes on the Performance of Solid‐State Batteries.” Advanced Energy Materials, vol. 11, no. 24, May. 2021, p. 2100654. https://doi.org/10.1002/aenm.202100654.

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Wiley

Journal

Advanced Energy Materials

Quartile SCImago

Quartile WOS

Impact factor

27.8

ISSN

16146832 (Print)
16146840 (Electronic)

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Janek, Jürgen