Advanced Energy Materials, volume 12, issue 25, pages 2200660
Super Long‐Cycling All‐Solid‐State Battery with Thin Li 6 PS 5 Cl‐Based Electrolyte
Sijie Liu
1
,
LE ZHOU
1
,
Jian Han
1
,
Kaihua Wen
1
,
Shundong Guan
1
,
Chuanjiao Xue
1
,
Zheng Zhang
1
,
Ben Xu
2
,
Yuanhua Lin
1
,
Yang Shen
1
,
Liangliang Li
1
,
Publication type: Journal Article
Publication date: 2022-05-06
Journal:
Advanced Energy Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 27.8
ISSN: 16146832, 16146840
General Materials Science
Renewable Energy, Sustainability and the Environment
Abstract
All-solid-state batteries (ASSBs) using sulfide electrolytes have attracted ever-increasing interest due to high ionic conductivity of the sulfides. Nevertheless, a thin, strong solid-state sulfide electrolyte membrane maintaining high ionic conductivity is highly desired for ASSBs. Here, a thin, flexible composite solid electrolyte membrane composed of argyrodite sulfide Li6PS5Cl and a polar poly(vinylidene fluoride-co-trifluoroethylene) (P(VDF-TrFE)) framework is prepared via an electrospinning-infiltration-hot-pressing method. The interaction between Li6PS5Cl and polar P(VDF-TrFE) ensures a high lithium-ion conductivity (≈1.2 mS cm–1) at room temperature and good mechanical ductility of the composite electrolyte membrane. The coin-type ASSB cells with the thin composite electrolyte membrane, a composite cathode of LiNbO3-coated LiNi0.8Co0.1Mn0.1O2 and Li6PS5Cl, and a lithium-indium anode, show super cycling performance, and the capacity retention is 92% after 1000 cycles and 71% even after 20 000 cycles at 1.0 mA cm–2 (i.e., 1.61 C) at room temperature. Moreover, pouch-type ASSB cells with a high mass loading of active materials are made to demonstrate the potential and feasibility in future commercial applications.
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Citations by publishers
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5
10
15
20
25
30
35
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Springer Nature
4 publications, 5.06%
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2 publications, 2.53%
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American Association for the Advancement of Science (AAAS)
1 publication, 1.27%
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The Electrochemical Society
1 publication, 1.27%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 1.27%
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5
10
15
20
25
30
35
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Liu S. et al. Super Long‐Cycling All‐Solid‐State Battery with Thin Li 6 PS 5 Cl‐Based Electrolyte // Advanced Energy Materials. 2022. Vol. 12. No. 25. p. 2200660.
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Liu S., ZHOU L., Han J., Wen K., Guan S., Xue C., Zhang Z., Xu B., Lin Y., Shen Y., Li L., Nan C. W. Super Long‐Cycling All‐Solid‐State Battery with Thin Li 6 PS 5 Cl‐Based Electrolyte // Advanced Energy Materials. 2022. Vol. 12. No. 25. p. 2200660.
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TY - JOUR
DO - 10.1002/aenm.202200660
UR - https://doi.org/10.1002/aenm.202200660
TI - Super Long‐Cycling All‐Solid‐State Battery with Thin Li 6 PS 5 Cl‐Based Electrolyte
T2 - Advanced Energy Materials
AU - Liu, Sijie
AU - Wen, Kaihua
AU - Guan, Shundong
AU - Xue, Chuanjiao
AU - Xu, Ben
AU - Lin, Yuanhua
AU - Li, Liangliang
AU - Nan, Ce Wen
AU - ZHOU, LE
AU - Han, Jian
AU - Zhang, Zheng
AU - Shen, Yang
PY - 2022
DA - 2022/05/06 00:00:00
PB - Wiley
SP - 2200660
IS - 25
VL - 12
SN - 1614-6832
SN - 1614-6840
ER -
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@article{2022_Liu,
author = {Sijie Liu and Kaihua Wen and Shundong Guan and Chuanjiao Xue and Ben Xu and Yuanhua Lin and Liangliang Li and Ce Wen Nan and LE ZHOU and Jian Han and Zheng Zhang and Yang Shen},
title = {Super Long‐Cycling All‐Solid‐State Battery with Thin Li 6 PS 5 Cl‐Based Electrolyte},
journal = {Advanced Energy Materials},
year = {2022},
volume = {12},
publisher = {Wiley},
month = {may},
url = {https://doi.org/10.1002/aenm.202200660},
number = {25},
pages = {2200660},
doi = {10.1002/aenm.202200660}
}
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MLA
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Liu, Sijie, et al. “Super Long‐Cycling All‐Solid‐State Battery with Thin Li 6 PS 5 Cl‐Based Electrolyte.” Advanced Energy Materials, vol. 12, no. 25, May. 2022, p. 2200660. https://doi.org/10.1002/aenm.202200660.