Advanced Energy Materials, pages 2202094

Sulfur Reduction Reaction in Lithium–Sulfur Batteries: Mechanisms, Catalysts, and Characterization

Lei Zhou ^{1, 2}

Dmitri L. Danilov ^{2, 3}

Fen Qiao ¹

Junfeng Wang ¹

Haitao Li ⁴

Rüdiger-A. Eichel ^{3, 5}

Peter H. L. Notten ^{2, 3, 6}

Hide authors affiliations Show authors affiliations: 6 affiliations

School of Energy and Power Engineering Jiangsu University Zhenjiang 212013 China |

Department of Chemical Engineering and Chemistry Department of Electrical Engineering Eindhoven University of Technology Eindhoven MB 5600 The Netherlands |

Institute of Energy and Climate Research Fundamental Electrochemistry (IEK‐9) Forschungszentrum Jülich D‐52425 Jülich Germany |

⁴

Institute for Energy Research School of Chemistry and Chemical Engineering Jiangsu University Zhenjiang 212013 China |

⁵

Institute of Physical Chemistry RWTH Aachen University D‐52074 Aachen Germany |

⁶

Centre for Clean Energy Technology University of Technology Sydney Broadway Sydney NSW 2007 Australia |

Publication type: Journal Article

Publication date: 2022-09-18

Wiley

Journal: Advanced Energy Materials

Quartile SCImago

Quartile WOS

Impact factor: 27.8

ISSN: 16146832, 16146840

DOI: 10.1002/aenm.202202094

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General Materials Science

Renewable Energy, Sustainability and the Environment

Abstract

Lithium–sulfur batteries are one of the most promising alternatives for advanced battery systems due to the merits of extraordinary theoretical specific energy density, abundant resources, environmental friendliness, and high safety. However, the sluggish sulfur reduction reaction (SRR) kinetics results in poor sulfur utilization, which seriously hampers the electrochemical performance of Li–S batteries. It is critical to reveal the underlying reaction mechanisms and accelerate the SRR kinetics. Herein, the critical issues of SRR in Li–S batteries are reviewed. The conversion mechanisms and reaction pathways of sulfur reduction are initially introduced to give an overview of the SRR. Subsequently, recent advances in catalyst materials that can accelerate the SRR kinetics are summarized in detail, including carbon, metal compounds, metals, and single atoms. Besides, various characterization approaches for SRR are discussed, which can be divided into three categories: electrochemical measurements, spectroscopic techniques, and theoretical calculations. Finally, the conclusion and outlook part gives a summary and proposes several key points for future investigations on the mechanisms of the SRR and catalyst activities. This review can provide cutting-edge insights into the SRR in Li–S batteries.

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Top-30

Citations by journals

	2 4 6 8 10
Small	Small, 10, 7.94% Small 10 publications, 7.94%
Advanced Functional Materials	Advanced Functional Materials, 9, 7.14% Advanced Functional Materials 9 publications, 7.14%
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ACS applied materials & interfaces	ACS applied materials & interfaces, 5, 3.97% ACS applied materials & interfaces 5 publications, 3.97%
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Angewandte Chemie	Angewandte Chemie, 4, 3.17% Angewandte Chemie 4 publications, 3.17%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 4, 3.17% Angewandte Chemie - International Edition 4 publications, 3.17%
Journal of Energy Chemistry	Journal of Energy Chemistry, 4, 3.17% Journal of Energy Chemistry 4 publications, 3.17%
Nanomaterials	Nanomaterials, 3, 2.38% Nanomaterials 3 publications, 2.38%
Advanced Science	Advanced Science, 3, 2.38% Advanced Science 3 publications, 2.38%
ACS Nano	ACS Nano, 3, 2.38% ACS Nano 3 publications, 2.38%
Advanced Materials	Advanced Materials, 3, 2.38% Advanced Materials 3 publications, 2.38%
Batteries	Batteries, 2, 1.59% Batteries 2 publications, 1.59%
Coordination Chemistry Reviews	Coordination Chemistry Reviews, 2, 1.59% Coordination Chemistry Reviews 2 publications, 1.59%
ACS Applied Energy Materials	ACS Applied Energy Materials, 2, 1.59% ACS Applied Energy Materials 2 publications, 1.59%
Materials Chemistry Frontiers	Materials Chemistry Frontiers, 2, 1.59% Materials Chemistry Frontiers 2 publications, 1.59%
Journal of the American Chemical Society	Journal of the American Chemical Society, 2, 1.59% Journal of the American Chemical Society 2 publications, 1.59%
ACS Sustainable Chemistry and Engineering	ACS Sustainable Chemistry and Engineering, 2, 1.59% ACS Sustainable Chemistry and Engineering 2 publications, 1.59%
ACS Applied Nano Materials	ACS Applied Nano Materials, 2, 1.59% ACS Applied Nano Materials 2 publications, 1.59%
Science China Materials	Science China Materials, 2, 1.59% Science China Materials 2 publications, 1.59%
Nature Chemical Engineering	Nature Chemical Engineering, 2, 1.59% Nature Chemical Engineering 2 publications, 1.59%
Journal of Energy Storage	Journal of Energy Storage, 2, 1.59% Journal of Energy Storage 2 publications, 1.59%
Nano-Micro Letters	Nano-Micro Letters, 1, 0.79% Nano-Micro Letters 1 publication, 0.79%
Applied Surface Science	Applied Surface Science, 1, 0.79% Applied Surface Science 1 publication, 0.79%
Transactions of Tianjin University	Transactions of Tianjin University, 1, 0.79% Transactions of Tianjin University 1 publication, 0.79%
Advanced Sustainable Systems	Advanced Sustainable Systems, 1, 0.79% Advanced Sustainable Systems 1 publication, 0.79%
Chemical Engineering Science	Chemical Engineering Science, 1, 0.79% Chemical Engineering Science 1 publication, 0.79%
Advanced Energy and Sustainability Research	Advanced Energy and Sustainability Research, 1, 0.79% Advanced Energy and Sustainability Research 1 publication, 0.79%
	2 4 6 8 10

Citations by publishers

	5 10 15 20 25 30 35 40 45
Wiley	Wiley, 42, 33.33% Wiley 42 publications, 33.33%
Elsevier	Elsevier, 40, 31.75% Elsevier 40 publications, 31.75%
American Chemical Society (ACS)	American Chemical Society (ACS), 19, 15.08% American Chemical Society (ACS) 19 publications, 15.08%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 8, 6.35% Multidisciplinary Digital Publishing Institute (MDPI) 8 publications, 6.35%
Springer Nature	Springer Nature, 7, 5.56% Springer Nature 7 publications, 5.56%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 3, 2.38% Royal Society of Chemistry (RSC) 3 publications, 2.38%
Tianjin Daxue/Tianjin University	Tianjin Daxue/Tianjin University, 1, 0.79% Tianjin Daxue/Tianjin University 1 publication, 0.79%
IOP Publishing	IOP Publishing, 1, 0.79% IOP Publishing 1 publication, 0.79%
OAE Publishing Inc.	OAE Publishing Inc., 1, 0.79% OAE Publishing Inc. 1 publication, 0.79%
Research Square Platform LLC	Research Square Platform LLC, 1, 0.79% Research Square Platform LLC 1 publication, 0.79%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.79% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.79%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 0.79% American Institute of Physics (AIP) 1 publication, 0.79%
The Electrochemical Society	The Electrochemical Society, 1, 0.79% The Electrochemical Society 1 publication, 0.79%
	5 10 15 20 25 30 35 40 45

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Zhou L. et al. Sulfur Reduction Reaction in Lithium–Sulfur Batteries: Mechanisms, Catalysts, and Characterization // Advanced Energy Materials. 2022. p. 2202094.

GOST all authors (up to 50) Copy

Zhou L., Danilov D. L., Qiao F., Wang J., Li H., Eichel R., Notten P. H. L. Sulfur Reduction Reaction in Lithium–Sulfur Batteries: Mechanisms, Catalysts, and Characterization // Advanced Energy Materials. 2022. p. 2202094.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1002/aenm.202202094

UR - https://doi.org/10.1002/aenm.202202094

TI - Sulfur Reduction Reaction in Lithium–Sulfur Batteries: Mechanisms, Catalysts, and Characterization

T2 - Advanced Energy Materials

AU - Zhou, Lei

AU - Danilov, Dmitri L.

AU - Qiao, Fen

AU - Wang, Junfeng

AU - Li, Haitao

AU - Eichel, Rüdiger-A.

AU - Notten, Peter H. L.

PY - 2022

DA - 2022/09/18 00:00:00

PB - Wiley

SP - 2202094

SN - 1614-6832

SN - 1614-6840

ER -

BibTex

Cite this

BibTex Copy

@article{2022_Zhou,

author = {Lei Zhou and Dmitri L. Danilov and Fen Qiao and Junfeng Wang and Haitao Li and Rüdiger-A. Eichel and Peter H. L. Notten},

title = {Sulfur Reduction Reaction in Lithium–Sulfur Batteries: Mechanisms, Catalysts, and Characterization},

journal = {Advanced Energy Materials},

year = {2022},

publisher = {Wiley},

month = {sep},

url = {https://doi.org/10.1002/aenm.202202094},

pages = {2202094},

doi = {10.1002/aenm.202202094}

}

Found error?

Publisher

Wiley

Journal

Advanced Energy Materials

Quartile SCImago

Quartile WOS

Impact factor

27.8

ISSN

16146832 (Print)
16146840 (Electronic)