volume 26 , issue 8 , pages 771-773

A 1-Oxa-2-nickela-5-cyclopentanone from Ethene and Carbon Dioxide: Preparation, Structure, and Reactivity

Heinz Hoberg ¹

Yolande Peres ¹

Carl Krüger ¹

Yi-Hung Tsay ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

Max‐Planck‐Institut für Kohlenforschung, Kaiser‐Wilhelm‐Platz 1, D‐4330 Mülheim a. d. Ruhr 1 (FRG) |

Publication type: Journal Article

Publication date: 1987-08-01

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DOI: 10.1002/anie.198707711

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General Chemistry

Catalysis

Abstract

Complex 1 is a key intermediate in the Ni0-promoted CC bond formation between alkenes and CO2; it contains 1,8-diazabicyclo[5.4.0]undec-7-ene (DBU) as ligand. The NiC bond of 1 can participate in further, regioselective insertion reactions with alkenes. The nickelacycle is thus a model complex for the study of Ni-catalyzed reactions.

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