volume 28
,
issue 9
,
pages 1216-1218
Asymmetric Oligomerization of Propene and 1-Butene with a Zirconocene/Alumoxane Catalyst
1
Institut für Technische und Makromolekulare Chemie der Universität, Bundesstrasse 45, D-2000 Hamburg 13 (FRG)
|
Publication type: Journal Article
Publication date: 1989-09-01
—
General Chemistry
Catalysis
Abstract
Approximately 80 % stereoselectivity in the creation of the second chiral center is observed during olefin oligomerization when chiral zirconocene complex (S)-1 together with methylalumoxane is used as catalyst. The oligomerization product mixture can be largely restricted to dimers through pentamers by appropriate choice of catalyst-to-monomer concentration. Relatively straight forward access is thereby provided to alkyl-substituted 1-alkenes such as 2 and 3, which could be of interest in the synthesis of pheromones and other modestly functionalized chiral compounds. [Zr(CH2-indenyl)2{O2CCH(OAc)Ph}2]
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102
Total citations:
102
Citations from 2025:
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(0.98%)