volume 54 issue 45 pages 13416-13419

A Neutral Silicon/Phosphorus Frustrated Lewis Pair

Publication typeJournal Article
Publication date2015-11-02
scimago Q1
wos Q1
SJR5.550
CiteScore27.6
Impact factor16.9
ISSN14337851, 15213773
General Chemistry
Catalysis
Abstract
Frustrated Lewis pairs (FLPs) have a great potential for activation of small molecules. Most known FLP systems are based on boron or aluminum atoms as acid functions, few on zinc, and only two on boron-isoelectronic silicenium cation systems. The first FLP system based on a neutral silane, (C2F5)3SiCH2P(tBu)2 (1), was prepared from (C2F5)3SiCl with C2F5 groups of very high electronegativity and LiCH2P(tBu)2. 1 is capable of cleaving hydrogen, and adds CO2 and SO2. Hydrogen splitting was confirmed by H/D scrambling reactions. The structures of 1, its CO2 and SO2 adducts, and a decomposition product with CO2 were elucidated by X-ray diffraction.
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GOST Copy
Waerder B. et al. A Neutral Silicon/Phosphorus Frustrated Lewis Pair // Angewandte Chemie - International Edition. 2015. Vol. 54. No. 45. pp. 13416-13419.
GOST all authors (up to 50) Copy
Waerder B., Pieper M., Körte L. A., Kinder T. A., Mix A., Neumann B., Stammler H., Mitzel N. W. A Neutral Silicon/Phosphorus Frustrated Lewis Pair // Angewandte Chemie - International Edition. 2015. Vol. 54. No. 45. pp. 13416-13419.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1002/anie.201504171
UR - https://doi.org/10.1002/anie.201504171
TI - A Neutral Silicon/Phosphorus Frustrated Lewis Pair
T2 - Angewandte Chemie - International Edition
AU - Waerder, Benedikt
AU - Pieper, Martin
AU - Körte, Leif A
AU - Kinder, Timo A
AU - Mix, A
AU - Neumann, Beate
AU - Stammler, Hans-Georg
AU - Mitzel, Norbert Werner
PY - 2015
DA - 2015/11/02
PB - Wiley
SP - 13416-13419
IS - 45
VL - 54
PMID - 26423202
SN - 1433-7851
SN - 1521-3773
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2015_Waerder,
author = {Benedikt Waerder and Martin Pieper and Leif A Körte and Timo A Kinder and A Mix and Beate Neumann and Hans-Georg Stammler and Norbert Werner Mitzel},
title = {A Neutral Silicon/Phosphorus Frustrated Lewis Pair},
journal = {Angewandte Chemie - International Edition},
year = {2015},
volume = {54},
publisher = {Wiley},
month = {nov},
url = {https://doi.org/10.1002/anie.201504171},
number = {45},
pages = {13416--13419},
doi = {10.1002/anie.201504171}
}
MLA
Cite this
MLA Copy
Waerder, Benedikt, et al. “A Neutral Silicon/Phosphorus Frustrated Lewis Pair.” Angewandte Chemie - International Edition, vol. 54, no. 45, Nov. 2015, pp. 13416-13419. https://doi.org/10.1002/anie.201504171.