volume 54 issue 47 pages 14017-14021

Visible‐Light‐Mediated Generation of Nitrogen‐Centered Radicals: Metal‐Free Hydroimination and Iminohydroxylation Cyclization Reactions

Publication typeJournal Article
Publication date2015-09-28
scimago Q1
wos Q1
SJR5.550
CiteScore27.6
Impact factor16.9
ISSN14337851, 15213773
General Chemistry
Catalysis
Abstract

The formation and use of iminyl radicals in novel and divergent hydroimination and iminohydroxylation cyclization reactions has been accomplished through the design of a new class of reactive O‐aryl oximes. Owing to their low reduction potentials, the inexpensive organic dye eosin Y could be used as the photocatalyst of the organocatalytic hydroimination reaction. Furthermore, reaction conditions for a unique iminohydroxylation were identified; visible‐light‐mediated electron transfer from novel electron donor–acceptor complexes of the oximes and Et3N was proposed as a key step of this process.

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GOST Copy
Davies J. et al. Visible‐Light‐Mediated Generation of Nitrogen‐Centered Radicals: Metal‐Free Hydroimination and Iminohydroxylation Cyclization Reactions // Angewandte Chemie - International Edition. 2015. Vol. 54. No. 47. pp. 14017-14021.
GOST all authors (up to 50) Copy
Davies J., Booth S. G., Essafi S., Dryfe R. A., Leonori D. Visible‐Light‐Mediated Generation of Nitrogen‐Centered Radicals: Metal‐Free Hydroimination and Iminohydroxylation Cyclization Reactions // Angewandte Chemie - International Edition. 2015. Vol. 54. No. 47. pp. 14017-14021.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1002/anie.201507641
UR - https://onlinelibrary.wiley.com/doi/10.1002/anie.201507641
TI - Visible‐Light‐Mediated Generation of Nitrogen‐Centered Radicals: Metal‐Free Hydroimination and Iminohydroxylation Cyclization Reactions
T2 - Angewandte Chemie - International Edition
AU - Davies, Jacob
AU - Booth, Samuel Guy
AU - Essafi, Stephanie
AU - Dryfe, Robert AW
AU - Leonori, Daniele
PY - 2015
DA - 2015/09/28
PB - Wiley
SP - 14017-14021
IS - 47
VL - 54
PMID - 26412046
SN - 1433-7851
SN - 1521-3773
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2015_Davies,
author = {Jacob Davies and Samuel Guy Booth and Stephanie Essafi and Robert AW Dryfe and Daniele Leonori},
title = {Visible‐Light‐Mediated Generation of Nitrogen‐Centered Radicals: Metal‐Free Hydroimination and Iminohydroxylation Cyclization Reactions},
journal = {Angewandte Chemie - International Edition},
year = {2015},
volume = {54},
publisher = {Wiley},
month = {sep},
url = {https://onlinelibrary.wiley.com/doi/10.1002/anie.201507641},
number = {47},
pages = {14017--14021},
doi = {10.1002/anie.201507641}
}
MLA
Cite this
MLA Copy
Davies, Jacob, et al. “Visible‐Light‐Mediated Generation of Nitrogen‐Centered Radicals: Metal‐Free Hydroimination and Iminohydroxylation Cyclization Reactions.” Angewandte Chemie - International Edition, vol. 54, no. 47, Sep. 2015, pp. 14017-14021. https://onlinelibrary.wiley.com/doi/10.1002/anie.201507641.