Single Lithium‐Ion Conducting Polymer Electrolytes Based on a Super‐Delocalized Polyanion
Qiang Ma
1
,
Heng Zhang
1
,
Chongwang Zhou
1
,
Liping Zheng
1
,
Pengfei Cheng
1
,
Jin Nie
1
,
Feng Wenfang
1
,
Yongsheng Hu
2
,
Hong Li
2
,
Xuejie Huang
2
,
Liquan Chen
2
,
Michel Armand
3
,
Zhibin Zhou
1
3
CIC energigune; Alava Technology Park, Albert Einstein; 4801510 MIÑANO Álava Spain
|
Publication type: Journal Article
Publication date: 2016-01-14
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
26840215
General Chemistry
Catalysis
Abstract
A novel single lithium‐ion (Li‐ion) conducting polymer electrolyte is presented that is composed of the lithium salt of a polyanion, poly[(4‐styrenesulfonyl)(trifluoromethyl(S‐trifluoromethylsulfonylimino)sulfonyl)imide] (PSsTFSI−), and high‐molecular‐weight poly(ethylene oxide) (PEO). The neat LiPSsTFSI ionomer displays a low glass‐transition temperature (44.3 °C; that is, strongly plasticizing effect). The complex of LiPSsTFSI/PEO exhibits a high Li‐ion transference number (tLi+=0.91) and is thermally stable up to 300 °C. Meanwhile, it exhibits a Li‐ion conductivity as high as 1.35×10−4 S cm−1 at 90 °C, which is comparable to that for the classic ambipolar LiTFSI/PEO SPEs at the same temperature. These outstanding properties of the LiPSsTFSI/PEO blended polymer electrolyte would make it promising as solid polymer electrolytes for Li batteries.
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445
Total citations:
445
Citations from 2024:
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(14%)
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Ma Q. et al. Single Lithium‐Ion Conducting Polymer Electrolytes Based on a Super‐Delocalized Polyanion // Angewandte Chemie - International Edition. 2016. Vol. 55. No. 7. pp. 2521-2525.
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Ma Q., Zhang H., Zhou C., Zheng L., Cheng P., Nie J., Wenfang F., Hu Y., Li H., Huang X., Chen L., Armand M., Zhou Z. Single Lithium‐Ion Conducting Polymer Electrolytes Based on a Super‐Delocalized Polyanion // Angewandte Chemie - International Edition. 2016. Vol. 55. No. 7. pp. 2521-2525.
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RIS
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TY - JOUR
DO - 10.1002/anie.201509299
UR - https://onlinelibrary.wiley.com/doi/10.1002/anie.201509299
TI - Single Lithium‐Ion Conducting Polymer Electrolytes Based on a Super‐Delocalized Polyanion
T2 - Angewandte Chemie - International Edition
AU - Ma, Qiang
AU - Zhang, Heng
AU - Zhou, Chongwang
AU - Zheng, Liping
AU - Cheng, Pengfei
AU - Nie, Jin
AU - Wenfang, Feng
AU - Hu, Yongsheng
AU - Li, Hong
AU - Huang, Xuejie
AU - Chen, Liquan
AU - Armand, Michel
AU - Zhou, Zhibin
PY - 2016
DA - 2016/01/14
PB - Wiley
SP - 2521-2525
IS - 7
VL - 55
PMID - 26840215
SN - 1433-7851
SN - 1521-3773
ER -
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BibTex (up to 50 authors)
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@article{2016_Ma,
author = {Qiang Ma and Heng Zhang and Chongwang Zhou and Liping Zheng and Pengfei Cheng and Jin Nie and Feng Wenfang and Yongsheng Hu and Hong Li and Xuejie Huang and Liquan Chen and Michel Armand and Zhibin Zhou},
title = {Single Lithium‐Ion Conducting Polymer Electrolytes Based on a Super‐Delocalized Polyanion},
journal = {Angewandte Chemie - International Edition},
year = {2016},
volume = {55},
publisher = {Wiley},
month = {jan},
url = {https://onlinelibrary.wiley.com/doi/10.1002/anie.201509299},
number = {7},
pages = {2521--2525},
doi = {10.1002/anie.201509299}
}
Cite this
MLA
Copy
Ma, Qiang, et al. “Single Lithium‐Ion Conducting Polymer Electrolytes Based on a Super‐Delocalized Polyanion.” Angewandte Chemie - International Edition, vol. 55, no. 7, Jan. 2016, pp. 2521-2525. https://onlinelibrary.wiley.com/doi/10.1002/anie.201509299.