Diverse Activation Modes in the Hydroboration of Aldehydes and Ketones with Germanium, Tin, and Lead Lewis Pairs.
Publication type: Journal Article
Publication date: 2016-12-02
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
27910186
General Chemistry
Catalysis
Abstract
Intramolecular germylene, stannylene, and plumbylene Lewis pairs were reacted with hexanal and yielded the cyclic addition products only with the germanium and tin reagents. In further reactivity studies, the hydroboration of aldehydes and ketones catalyzed by intramolecular germylene, stannylene, and plumbylene Lewis pairs was studied. In the case of the cyclic germylene Lewis pair, the product of the oxidative addition of pinacolborane at the germylene moiety was observed. According to stoichiometric as well as catalytic experiments, the intramolecular germylene Lewis pair acts as a catalyst in the hydroboration of aldehydes and ketones. The homologous stannylene Lewis pair forms a reactive tin hydride during the catalysis, which can also act as a catalyst in this transformation.
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Citations from 2025:
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GOST
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Schneider J. et al. Diverse Activation Modes in the Hydroboration of Aldehydes and Ketones with Germanium, Tin, and Lead Lewis Pairs. // Angewandte Chemie - International Edition. 2016. Vol. 56. No. 1. pp. 333-337.
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Schneider J., Sindlinger C. P., Freitag S. M., Schubert H., Wesemann L. Diverse Activation Modes in the Hydroboration of Aldehydes and Ketones with Germanium, Tin, and Lead Lewis Pairs. // Angewandte Chemie - International Edition. 2016. Vol. 56. No. 1. pp. 333-337.
Cite this
RIS
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TY - JOUR
DO - 10.1002/anie.201609155
UR - https://doi.org/10.1002/anie.201609155
TI - Diverse Activation Modes in the Hydroboration of Aldehydes and Ketones with Germanium, Tin, and Lead Lewis Pairs.
T2 - Angewandte Chemie - International Edition
AU - Schneider, Julia
AU - Sindlinger, Christian P.
AU - Freitag, Sarah M
AU - Schubert, Hartmut
AU - Wesemann, Lars
PY - 2016
DA - 2016/12/02
PB - Wiley
SP - 333-337
IS - 1
VL - 56
PMID - 27910186
SN - 1433-7851
SN - 1521-3773
ER -
Cite this
BibTex (up to 50 authors)
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@article{2016_Schneider,
author = {Julia Schneider and Christian P. Sindlinger and Sarah M Freitag and Hartmut Schubert and Lars Wesemann},
title = {Diverse Activation Modes in the Hydroboration of Aldehydes and Ketones with Germanium, Tin, and Lead Lewis Pairs.},
journal = {Angewandte Chemie - International Edition},
year = {2016},
volume = {56},
publisher = {Wiley},
month = {dec},
url = {https://doi.org/10.1002/anie.201609155},
number = {1},
pages = {333--337},
doi = {10.1002/anie.201609155}
}
Cite this
MLA
Copy
Schneider, Julia, et al. “Diverse Activation Modes in the Hydroboration of Aldehydes and Ketones with Germanium, Tin, and Lead Lewis Pairs..” Angewandte Chemie - International Edition, vol. 56, no. 1, Dec. 2016, pp. 333-337. https://doi.org/10.1002/anie.201609155.