Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels
Lu Lu
1, 2
,
Xiaofu Sun
1, 2
,
Ying Sun
1
,
dexin Yang
1, 2
,
Peng Wu
3
,
Bin Zhang
1, 2
,
Jianling Zhang
1, 2
,
Buxing Han
1, 2
Publication type: Journal Article
Publication date: 2018-10-02
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
30152923
General Chemistry
Catalysis
Abstract
Electrochemical reduction of CO2 to CH3 OH is of great interest. Aerogels have fine inorganic superstructure with high porosity and are known to be exceptional materials. Now a Pd-Cu bimetallic aerogel electrocatalyst has been developed for conversion of CO2 into CH3 OH. The current density and Faradaic efficiency of CH3 OH can be as high as 31.8 mA cm-2 and 80.0 % over the Pd83 Cu17 aerogel at a very low overpotential (0.24 V). The superior performance of the electrocatalyst results from efficient adsorption and stabilization of the CO2 radical anion, high Pd0 /PdII and CuI +Cu0 /CuII ratios, and sufficient Pd/Cu grain boundaries of aerogel nanochains.
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292
Total citations:
292
Citations from 2024:
80
(27.4%)
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GOST
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Lu L. et al. Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels // Angewandte Chemie - International Edition. 2018. Vol. 57. No. 43. pp. 14149-14153.
GOST all authors (up to 50)
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Lu L., Sun X., Sun Y., Yang D., Wu P., Zhang B., Zhang J., Han B. Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels // Angewandte Chemie - International Edition. 2018. Vol. 57. No. 43. pp. 14149-14153.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1002/anie.201808964
UR - https://doi.org/10.1002/anie.201808964
TI - Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels
T2 - Angewandte Chemie - International Edition
AU - Lu, Lu
AU - Sun, Xiaofu
AU - Sun, Ying
AU - Yang, dexin
AU - Wu, Peng
AU - Zhang, Bin
AU - Zhang, Jianling
AU - Han, Buxing
PY - 2018
DA - 2018/10/02
PB - Wiley
SP - 14149-14153
IS - 43
VL - 57
PMID - 30152923
SN - 1433-7851
SN - 1521-3773
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2018_Lu,
author = {Lu Lu and Xiaofu Sun and Ying Sun and dexin Yang and Peng Wu and Bin Zhang and Jianling Zhang and Buxing Han},
title = {Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels},
journal = {Angewandte Chemie - International Edition},
year = {2018},
volume = {57},
publisher = {Wiley},
month = {oct},
url = {https://doi.org/10.1002/anie.201808964},
number = {43},
pages = {14149--14153},
doi = {10.1002/anie.201808964}
}
Cite this
MLA
Copy
Lu, Lu, et al. “Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels.” Angewandte Chemie - International Edition, vol. 57, no. 43, Oct. 2018, pp. 14149-14153. https://doi.org/10.1002/anie.201808964.