Angewandte Chemie - International Edition, volume 57, issue 43, pages 14149-14153
Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels
Lu Lu
1, 2
,
Xiaofu Sun
1, 2
,
Ying Sun
1
,
dexin Yang
1, 2
,
Peng Wu
3
,
Bin Zhang
1, 2
,
Jianling Zhang
1, 2
,
Buxing Han
1, 2
Publication type: Journal Article
Publication date: 2018-10-02
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 16.6
ISSN: 14337851, 15213773
General Chemistry
Catalysis
Abstract
Electrochemical reduction of CO2 to CH3 OH is of great interest. Aerogels have fine inorganic superstructure with high porosity and are known to be exceptional materials. Now a Pd-Cu bimetallic aerogel electrocatalyst has been developed for conversion of CO2 into CH3 OH. The current density and Faradaic efficiency of CH3 OH can be as high as 31.8 mA cm-2 and 80.0 % over the Pd83 Cu17 aerogel at a very low overpotential (0.24 V). The superior performance of the electrocatalyst results from efficient adsorption and stabilization of the CO2 radical anion, high Pd0 /PdII and CuI +Cu0 /CuII ratios, and sufficient Pd/Cu grain boundaries of aerogel nanochains.
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Lu L. et al. Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels // Angewandte Chemie - International Edition. 2018. Vol. 57. No. 43. pp. 14149-14153.
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Lu L., Sun X., Sun Y., Yang D., Wu P., Zhang B., Zhang J., Han B. Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels // Angewandte Chemie - International Edition. 2018. Vol. 57. No. 43. pp. 14149-14153.
Cite this
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TY - JOUR
DO - 10.1002/anie.201808964
UR - https://doi.org/10.1002/anie.201808964
TI - Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels
T2 - Angewandte Chemie - International Edition
AU - Yang, dexin
AU - Zhang, Jianling
AU - Sun, Xiaofu
AU - Han, Buxing
AU - Lu, Lu
AU - Sun, Ying
AU - Wu, Peng
AU - Zhang, Bin
PY - 2018
DA - 2018/10/02
PB - Wiley
SP - 14149-14153
IS - 43
VL - 57
SN - 1433-7851
SN - 1521-3773
ER -
Cite this
BibTex
Copy
@article{2018_Lu,
author = {dexin Yang and Jianling Zhang and Xiaofu Sun and Buxing Han and Lu Lu and Ying Sun and Peng Wu and Bin Zhang},
title = {Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels},
journal = {Angewandte Chemie - International Edition},
year = {2018},
volume = {57},
publisher = {Wiley},
month = {oct},
url = {https://doi.org/10.1002/anie.201808964},
number = {43},
pages = {14149--14153},
doi = {10.1002/anie.201808964}
}
Cite this
MLA
Copy
Lu, Lu, et al. “Highly Efficient Electroreduction of CO2to Methanol on Palladium-Copper Bimetallic Aerogels.” Angewandte Chemie - International Edition, vol. 57, no. 43, Oct. 2018, pp. 14149-14153. https://doi.org/10.1002/anie.201808964.