Angewandte Chemie - International Edition, volume 58, issue 12, pages 3804-3808

Adjusting the Reduction Potential of Electrons by Quantum Confinement for Selective Photoreduction of CO 2 to Methanol

Publication typeJournal Article
Publication date2019-03-18
scimago Q1
wos Q1
SJR5.300
CiteScore26.6
Impact factor16.1
ISSN14337851, 15213773
General Chemistry
Catalysis
Abstract
The production of CH3 OH from the photocatalytic CO2 reduction reaction (PCRR) presents a promising route for the clean utilization of renewable resources, but charge recombination, an unsatisfying stability and a poor selectivity limit its practical application. In this paper, we present the design and fabrication of 0D/2D materials with polymeric C3 N4 nanosheets and CdSe quantum dots (QDs) to enhance the separation and reduce the diffusion length of charge carriers. The rapid outflow of carriers also restrains self-corrosion and consequently enhances the stability. Furthermore, based on quantum confinement effects of the QDs, the energy of the electrons could be adjusted to a level that inhibits the hydrogen evolution reaction (HER, the main competitive reaction to PCRR) and improves the selectivity and activity for CH3 OH production from the PCRR. The band structures of photocatalysts with various CdSe particle sizes were also investigated quantitatively to establish the relationship between the band energy and the photocatalytic performance.
Found 
Found 

Top-30

Journals

2
4
6
8
10
12
Chemical Engineering Journal
12 publications, 8.45%
ACS Catalysis
7 publications, 4.93%
Angewandte Chemie
5 publications, 3.52%
Angewandte Chemie - International Edition
5 publications, 3.52%
Small
5 publications, 3.52%
Applied Catalysis B: Environmental
4 publications, 2.82%
Chemistry - A European Journal
4 publications, 2.82%
Journal of Materials Chemistry A
4 publications, 2.82%
Nanoscale
4 publications, 2.82%
Applied Surface Science
3 publications, 2.11%
Carbon
3 publications, 2.11%
Journal of Colloid and Interface Science
3 publications, 2.11%
Advanced Materials
3 publications, 2.11%
Solar RRL
3 publications, 2.11%
Advanced Functional Materials
2 publications, 1.41%
Chinese Journal of Catalysis
2 publications, 1.41%
Catalysts
2 publications, 1.41%
Catalysis Letters
2 publications, 1.41%
Nano Research
2 publications, 1.41%
Journal of Environmental Chemical Engineering
2 publications, 1.41%
Advanced Energy Materials
2 publications, 1.41%
ACS applied materials & interfaces
2 publications, 1.41%
Journal of the American Chemical Society
2 publications, 1.41%
ACS Nano
2 publications, 1.41%
Sustainable Energy and Fuels
2 publications, 1.41%
EES Catalysis
2 publications, 1.41%
ChemCatChem
2 publications, 1.41%
Physical Chemistry Chemical Physics
2 publications, 1.41%
Industrial & Engineering Chemistry Research
2 publications, 1.41%
Journal of Materials Science: Materials in Electronics
1 publication, 0.7%
2
4
6
8
10
12

Publishers

5
10
15
20
25
30
35
40
45
50
Elsevier
47 publications, 33.1%
Wiley
36 publications, 25.35%
Royal Society of Chemistry (RSC)
21 publications, 14.79%
American Chemical Society (ACS)
20 publications, 14.08%
Springer Nature
13 publications, 9.15%
MDPI
4 publications, 2.82%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 0.7%
5
10
15
20
25
30
35
40
45
50
  • We do not take into account publications without a DOI.
  • Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
  • Statistics recalculated weekly.

Are you a researcher?

Create a profile to get free access to personal recommendations for colleagues and new articles.
Metrics
Share
Cite this
GOST |
Cite this
GOST Copy
Li A. et al. Adjusting the Reduction Potential of Electrons by Quantum Confinement for Selective Photoreduction of CO 2 to Methanol // Angewandte Chemie - International Edition. 2019. Vol. 58. No. 12. pp. 3804-3808.
GOST all authors (up to 50) Copy
Li A., Wang T., Li C., Huang Z., Luo Z., Gong J. Adjusting the Reduction Potential of Electrons by Quantum Confinement for Selective Photoreduction of CO 2 to Methanol // Angewandte Chemie - International Edition. 2019. Vol. 58. No. 12. pp. 3804-3808.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1002/anie.201812773
UR - https://doi.org/10.1002/anie.201812773
TI - Adjusting the Reduction Potential of Electrons by Quantum Confinement for Selective Photoreduction of CO 2 to Methanol
T2 - Angewandte Chemie - International Edition
AU - Li, Ang
AU - Wang, Tuo
AU - Li, Chengcheng
AU - Huang, Zhiqi
AU - Luo, Zhibin
AU - Gong, Jinlong
PY - 2019
DA - 2019/03/18
PB - Wiley
SP - 3804-3808
IS - 12
VL - 58
SN - 1433-7851
SN - 1521-3773
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2019_Li,
author = {Ang Li and Tuo Wang and Chengcheng Li and Zhiqi Huang and Zhibin Luo and Jinlong Gong},
title = {Adjusting the Reduction Potential of Electrons by Quantum Confinement for Selective Photoreduction of CO 2 to Methanol},
journal = {Angewandte Chemie - International Edition},
year = {2019},
volume = {58},
publisher = {Wiley},
month = {mar},
url = {https://doi.org/10.1002/anie.201812773},
number = {12},
pages = {3804--3808},
doi = {10.1002/anie.201812773}
}
MLA
Cite this
MLA Copy
Li, Ang, et al. “Adjusting the Reduction Potential of Electrons by Quantum Confinement for Selective Photoreduction of CO 2 to Methanol.” Angewandte Chemie - International Edition, vol. 58, no. 12, Mar. 2019, pp. 3804-3808. https://doi.org/10.1002/anie.201812773.
Found error?