Reverse Arene Sandwich Structures Based upon π‐Hole⋅⋅⋅[M II ] (d 8 M=Pt, Pd) Interactions, where Positively Charged Metal Centers Play the Role of a Nucleophile
Тип публикации: Journal Article
Дата публикации: 2019-02-14
scimago Q1
wos Q1
БС1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
30667579
General Chemistry
Catalysis
Краткое описание
The complexes [Pt(tpp)] (H2tpp=tetraphenylporphyrin), [M(acac)2] (M=Pd, Pt, Hacac=acetylacetone), and [Pd(ba)2] (Hba=benzoylacetone) were co‐crystallized with highly electron‐deficient arene systems to form reverse arene sandwich structures built by π‐hole⋅⋅⋅[MII] (d8M=Pt, Pd) interactions. The adduct [Pt(tpp)]⋅2 C6F6 is monomeric, whereas the diketonate 1:1 adducts form columnar infinity 1D‐stack assembled by simultaneous action of both π‐hole⋅⋅⋅[MII] and C⋅⋅⋅F interactions. The reverse sandwiches are based on noncovalent interactions and calculated ESP distributions indicate that in π‐hole⋅⋅⋅[MII] contacts, [MII] plays the role of a nucleophile.
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Rozhkov A. A. et al. Reverse Arene Sandwich Structures Based upon π‐Hole⋅⋅⋅[M II ] (d 8 M=Pt, Pd) Interactions, where Positively Charged Metal Centers Play the Role of a Nucleophile // Angewandte Chemie - International Edition. 2019. Vol. 58. No. 13. pp. 4164-4168.
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Rozhkov A. A., Krykova M. A., Ivanov D. M., Novikov A. S., Sinelshchikova A., Volostnykh M. V., Konovalov M. A., Grigoriev M. S., Gorbunova Y. G., Kukushkin V. Y. Reverse Arene Sandwich Structures Based upon π‐Hole⋅⋅⋅[M II ] (d 8 M=Pt, Pd) Interactions, where Positively Charged Metal Centers Play the Role of a Nucleophile // Angewandte Chemie - International Edition. 2019. Vol. 58. No. 13. pp. 4164-4168.
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TY - JOUR
DO - 10.1002/anie.201814062
UR - https://onlinelibrary.wiley.com/doi/10.1002/anie.201814062
TI - Reverse Arene Sandwich Structures Based upon π‐Hole⋅⋅⋅[M II ] (d 8 M=Pt, Pd) Interactions, where Positively Charged Metal Centers Play the Role of a Nucleophile
T2 - Angewandte Chemie - International Edition
AU - Rozhkov, Anton Alekseevich
AU - Krykova, Mariya A
AU - Ivanov, Daniil M
AU - Novikov, Alexander S.
AU - Sinelshchikova, Anna
AU - Volostnykh, Marina V
AU - Konovalov, Mikhail A
AU - Grigoriev, Mikhail S.
AU - Gorbunova, Yulia G.
AU - Kukushkin, Vadim Yu.
PY - 2019
DA - 2019/02/14
PB - Wiley
SP - 4164-4168
IS - 13
VL - 58
PMID - 30667579
SN - 1433-7851
SN - 1521-3773
ER -
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@article{2019_Rozhkov,
author = {Anton Alekseevich Rozhkov and Mariya A Krykova and Daniil M Ivanov and Alexander S. Novikov and Anna Sinelshchikova and Marina V Volostnykh and Mikhail A Konovalov and Mikhail S. Grigoriev and Yulia G. Gorbunova and Vadim Yu. Kukushkin},
title = {Reverse Arene Sandwich Structures Based upon π‐Hole⋅⋅⋅[M II ] (d 8 M=Pt, Pd) Interactions, where Positively Charged Metal Centers Play the Role of a Nucleophile},
journal = {Angewandte Chemie - International Edition},
year = {2019},
volume = {58},
publisher = {Wiley},
month = {feb},
url = {https://onlinelibrary.wiley.com/doi/10.1002/anie.201814062},
number = {13},
pages = {4164--4168},
doi = {10.1002/anie.201814062}
}
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Rozhkov, Anton Alekseevich, et al. “Reverse Arene Sandwich Structures Based upon π‐Hole⋅⋅⋅[M II ] (d 8 M=Pt, Pd) Interactions, where Positively Charged Metal Centers Play the Role of a Nucleophile.” Angewandte Chemie - International Edition, vol. 58, no. 13, Feb. 2019, pp. 4164-4168. https://onlinelibrary.wiley.com/doi/10.1002/anie.201814062.