A Supramolecular Artificial Light‐Harvesting System with Two‐Step Sequential Energy Transfer for Photochemical Catalysis
Min Hao
1
,
Guangping Sun
1
,
Minzan Zuo
1
,
Zuqiang Xu
1
,
Yuan Chen
1
,
Xiao-Yu Hu
1, 2
,
Leyong Wang
1, 3
Publication type: Journal Article
Publication date: 2019-11-14
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
31625651
General Chemistry
Catalysis
Abstract
An artificial light-harvesting system with sequential energy-transfer process was fabricated based on a supramolecular strategy. Self-assembled from the host-guest complex formed by water-soluble pillar[5]arene (WP5), a bola-type tetraphenylethylene-functionalized dialkyl ammonium derivative (TPEDA), and two fluorescent dyes, Eosin Y (ESY) and Nile Red (NiR), the supramolecular vesicles achieve efficient energy transfer from the AIE guest TPEDA to ESY. ESY can function as a relay to further transfer the energy to the second acceptor NiR and realize a two-step sequential energy-transfer process with good efficiency. By tuning the donor/acceptor ratio, bright white light emission can be successfully achieved with a CIE coordinate of (0.33, 0.33). To better mimic natural photosynthesis and make full use of the harvested energy, the WP5⊃TPEDA-ESY-NiR system can be utilized as a nanoreactor: photocatalyzed dehalogenation of α-bromoacetophenone was realized with 96 % yield in aqueous medium.
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287
Total citations:
287
Citations from 2024:
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(33.8%)
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Hao M. et al. A Supramolecular Artificial Light‐Harvesting System with Two‐Step Sequential Energy Transfer for Photochemical Catalysis // Angewandte Chemie - International Edition. 2019. Vol. 59. No. 25. pp. 10095-10100.
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Hao M., Sun G., Zuo M., Xu Z., Chen Y., Hu X., Wang L. A Supramolecular Artificial Light‐Harvesting System with Two‐Step Sequential Energy Transfer for Photochemical Catalysis // Angewandte Chemie - International Edition. 2019. Vol. 59. No. 25. pp. 10095-10100.
Cite this
RIS
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TY - JOUR
DO - 10.1002/anie.201912654
UR - https://doi.org/10.1002/anie.201912654
TI - A Supramolecular Artificial Light‐Harvesting System with Two‐Step Sequential Energy Transfer for Photochemical Catalysis
T2 - Angewandte Chemie - International Edition
AU - Hao, Min
AU - Sun, Guangping
AU - Zuo, Minzan
AU - Xu, Zuqiang
AU - Chen, Yuan
AU - Hu, Xiao-Yu
AU - Wang, Leyong
PY - 2019
DA - 2019/11/14
PB - Wiley
SP - 10095-10100
IS - 25
VL - 59
PMID - 31625651
SN - 1433-7851
SN - 1521-3773
ER -
Cite this
BibTex (up to 50 authors)
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@article{2019_Hao,
author = {Min Hao and Guangping Sun and Minzan Zuo and Zuqiang Xu and Yuan Chen and Xiao-Yu Hu and Leyong Wang},
title = {A Supramolecular Artificial Light‐Harvesting System with Two‐Step Sequential Energy Transfer for Photochemical Catalysis},
journal = {Angewandte Chemie - International Edition},
year = {2019},
volume = {59},
publisher = {Wiley},
month = {nov},
url = {https://doi.org/10.1002/anie.201912654},
number = {25},
pages = {10095--10100},
doi = {10.1002/anie.201912654}
}
Cite this
MLA
Copy
Hao, Min, et al. “A Supramolecular Artificial Light‐Harvesting System with Two‐Step Sequential Energy Transfer for Photochemical Catalysis.” Angewandte Chemie - International Edition, vol. 59, no. 25, Nov. 2019, pp. 10095-10100. https://doi.org/10.1002/anie.201912654.