Unraveling the Impact of Gold(I)–Thiolate Motifs on the Aggregation‐Induced Emission of Gold Nanoclusters
Zhennan Wu
1
,
Qiaofeng Yao
1
,
Osburg Jin Huang Chai
1
,
Nan Ding
2
,
Wen Xu
2
,
Shuang-Quan Zang
3
,
Jianping Xie
1, 4
Publication type: Journal Article
Publication date: 2020-02-28
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
32011796
General Chemistry
Catalysis
Abstract
Aggregation-induced emission (AIE) provides an efficient strategy to synthesize highly luminescent metal nanoclusters (NCs), however, rational control of emission energy and intensity of metal NCs is still challenging. This communication reveals the impact of surface AuI -thiolate motifs on the AIE properties of Au NCs, by employing a series of water-soluble glutathione (GSH)-coordinated Au complexes and NCs as a model ([Au10 SR10 ], [Au15 SR13 ], [Au18 SR14 ], and [Au25 SR18 ]- , SR=thiolate ligand). Spectroscopic investigations show that the emission wavelength of Au NCs is adjustable from visible to the near-infrared II (NIR-II) region by controlling the length of the AuI -SR motifs on the NC surface. Decreasing the length of AuI -SR motifs also changes the origin of cluster luminescence from AIE-type phosphorescence to Au0 -core-dictated fluorescence. This effect becomes more prominent when the degree of aggregation of Au NCs increases in solution.
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271
Total citations:
271
Citations from 2025:
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(16.97%)
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Wu Z. et al. Unraveling the Impact of Gold(I)–Thiolate Motifs on the Aggregation‐Induced Emission of Gold Nanoclusters // Angewandte Chemie - International Edition. 2020. Vol. 59. No. 25. pp. 9934-9939.
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Wu Z., Yao Q., Chai O. J. H., Ding N., Xu W., Zang S., Xie J. Unraveling the Impact of Gold(I)–Thiolate Motifs on the Aggregation‐Induced Emission of Gold Nanoclusters // Angewandte Chemie - International Edition. 2020. Vol. 59. No. 25. pp. 9934-9939.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1002/anie.201916675
UR - https://doi.org/10.1002/anie.201916675
TI - Unraveling the Impact of Gold(I)–Thiolate Motifs on the Aggregation‐Induced Emission of Gold Nanoclusters
T2 - Angewandte Chemie - International Edition
AU - Wu, Zhennan
AU - Yao, Qiaofeng
AU - Chai, Osburg Jin Huang
AU - Ding, Nan
AU - Xu, Wen
AU - Zang, Shuang-Quan
AU - Xie, Jianping
PY - 2020
DA - 2020/02/28
PB - Wiley
SP - 9934-9939
IS - 25
VL - 59
PMID - 32011796
SN - 1433-7851
SN - 1521-3773
ER -
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@article{2020_Wu,
author = {Zhennan Wu and Qiaofeng Yao and Osburg Jin Huang Chai and Nan Ding and Wen Xu and Shuang-Quan Zang and Jianping Xie},
title = {Unraveling the Impact of Gold(I)–Thiolate Motifs on the Aggregation‐Induced Emission of Gold Nanoclusters},
journal = {Angewandte Chemie - International Edition},
year = {2020},
volume = {59},
publisher = {Wiley},
month = {feb},
url = {https://doi.org/10.1002/anie.201916675},
number = {25},
pages = {9934--9939},
doi = {10.1002/anie.201916675}
}
Cite this
MLA
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Wu, Zhennan, et al. “Unraveling the Impact of Gold(I)–Thiolate Motifs on the Aggregation‐Induced Emission of Gold Nanoclusters.” Angewandte Chemie - International Edition, vol. 59, no. 25, Feb. 2020, pp. 9934-9939. https://doi.org/10.1002/anie.201916675.