Angewandte Chemie - International Edition, volume 60, issue 17, pages 9650-9659
Lewis Acid Strength of Interfacial Metal Sites Drives CH 3 OH Selectivity and Formation Rates on Cu‐Based CO 2 Hydrogenation Catalysts
Publication type: Journal Article
Publication date: 2021-03-18
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 16.6
ISSN: 14337851, 15213773
General Chemistry
Catalysis
Abstract
Cu nanoparticles, dispersed on supports decorated with isolated group IV and V metal centers on SiO2, catalyze the selective hydrogenation of CO2 to CH3OH. The promotion of CH3OH formation rates and selectivity correlates with the Lewis acid strength of the group IV and V dopants, which stabilize surface intermediates at the periphery of Cu nanoparticles.
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Noh G. et al. Lewis Acid Strength of Interfacial Metal Sites Drives CH 3 OH Selectivity and Formation Rates on Cu‐Based CO 2 Hydrogenation Catalysts // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 17. pp. 9650-9659.
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Noh G., Lam E., Bregante D. T., Meyet J., Šot P., Flaherty D. H., Copéret C. Lewis Acid Strength of Interfacial Metal Sites Drives CH 3 OH Selectivity and Formation Rates on Cu‐Based CO 2 Hydrogenation Catalysts // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 17. pp. 9650-9659.
Cite this
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TY - JOUR
DO - 10.1002/anie.202100672
UR - https://doi.org/10.1002/anie.202100672
TI - Lewis Acid Strength of Interfacial Metal Sites Drives CH 3 OH Selectivity and Formation Rates on Cu‐Based CO 2 Hydrogenation Catalysts
T2 - Angewandte Chemie - International Edition
AU - Noh, Gina
AU - Lam, Erwin
AU - Bregante, Daniel T
AU - Meyet, Jordan
AU - Šot, Petr
AU - Flaherty, David H.
AU - Copéret, Christophe
PY - 2021
DA - 2021/03/18
PB - Wiley
SP - 9650-9659
IS - 17
VL - 60
SN - 1433-7851
SN - 1521-3773
ER -
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@article{2021_Noh,
author = {Gina Noh and Erwin Lam and Daniel T Bregante and Jordan Meyet and Petr Šot and David H. Flaherty and Christophe Copéret},
title = {Lewis Acid Strength of Interfacial Metal Sites Drives CH 3 OH Selectivity and Formation Rates on Cu‐Based CO 2 Hydrogenation Catalysts},
journal = {Angewandte Chemie - International Edition},
year = {2021},
volume = {60},
publisher = {Wiley},
month = {mar},
url = {https://doi.org/10.1002/anie.202100672},
number = {17},
pages = {9650--9659},
doi = {10.1002/anie.202100672}
}
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Noh, Gina, et al. “Lewis Acid Strength of Interfacial Metal Sites Drives CH 3 OH Selectivity and Formation Rates on Cu‐Based CO 2 Hydrogenation Catalysts.” Angewandte Chemie - International Edition, vol. 60, no. 17, Mar. 2021, pp. 9650-9659. https://doi.org/10.1002/anie.202100672.