Electrocatalytic Activation of Donor–Acceptor Cyclopropanes and Cyclobutanes: An Alternative C(sp 3 )−C(sp 3 ) Cleavage Mode
Simon Kolb
1
,
Martin Petzold
1
,
Felix Brandt
2
,
Peter G. Jones
3
,
Christoph R Jacob
2
,
Daniel B. Werz
1
Publication type: Journal Article
Publication date: 2021-06-16
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
33890714
General Chemistry
Catalysis
Abstract
The first electrochemical activation of donor–acceptor (D–A) cyclopropanes and D–A cyclobutanes has been applied for the formal insertion of molecular oxygen into these compounds. C(sp3)−C(sp3) cleavage of the ring moieties was achieved either by direct anodic electrolysis or by utilizing a DDQ-assisted electrochemical strategy. Quantum-chemical calculations and supportive experiments provided mechanistic understanding of the electrocatalytic process.
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94
Total citations:
94
Citations from 2025:
16
(17.02%)
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GOST
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Kolb S. et al. Electrocatalytic Activation of Donor–Acceptor Cyclopropanes and Cyclobutanes: An Alternative C(sp 3 )−C(sp 3 ) Cleavage Mode // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 29. pp. 15928-15934.
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Kolb S., Petzold M., Brandt F., Jones P. G., Jacob C. R., Werz D. B. Electrocatalytic Activation of Donor–Acceptor Cyclopropanes and Cyclobutanes: An Alternative C(sp 3 )−C(sp 3 ) Cleavage Mode // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 29. pp. 15928-15934.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1002/anie.202101477
UR - https://doi.org/10.1002/anie.202101477
TI - Electrocatalytic Activation of Donor–Acceptor Cyclopropanes and Cyclobutanes: An Alternative C(sp 3 )−C(sp 3 ) Cleavage Mode
T2 - Angewandte Chemie - International Edition
AU - Kolb, Simon
AU - Petzold, Martin
AU - Brandt, Felix
AU - Jones, Peter G.
AU - Jacob, Christoph R
AU - Werz, Daniel B.
PY - 2021
DA - 2021/06/16
PB - Wiley
SP - 15928-15934
IS - 29
VL - 60
PMID - 33890714
SN - 1433-7851
SN - 1521-3773
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2021_Kolb,
author = {Simon Kolb and Martin Petzold and Felix Brandt and Peter G. Jones and Christoph R Jacob and Daniel B. Werz},
title = {Electrocatalytic Activation of Donor–Acceptor Cyclopropanes and Cyclobutanes: An Alternative C(sp 3 )−C(sp 3 ) Cleavage Mode},
journal = {Angewandte Chemie - International Edition},
year = {2021},
volume = {60},
publisher = {Wiley},
month = {jun},
url = {https://doi.org/10.1002/anie.202101477},
number = {29},
pages = {15928--15934},
doi = {10.1002/anie.202101477}
}
Cite this
MLA
Copy
Kolb, Simon, et al. “Electrocatalytic Activation of Donor–Acceptor Cyclopropanes and Cyclobutanes: An Alternative C(sp 3 )−C(sp 3 ) Cleavage Mode.” Angewandte Chemie - International Edition, vol. 60, no. 29, Jun. 2021, pp. 15928-15934. https://doi.org/10.1002/anie.202101477.